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Ultrafast Transport of Laser-Excited Spin-Polarized Carriers inAu/Fe/MgO(001)

Open access
Melnikov, Alexey, Razdolski, Ilya, Wehling, Tim O., Papaioannou, Evangelos Th., Roddatis, Vladimir, Fumagalli, Paul, Aktsipetrov, Oleg, Lichtenstein, Alexander I., Bovensiepen, Uwe·2011·Physical Review Letters

Abstract

Hot carrier-induced spin dynamics is analyzed in epitaxial Au/Fe/MgO(001) by a time domain approach. We excite a spin current pulse in Fe by 35 fs laser pulses. The transient spin polarization, which is probed at the Au surface by optical second harmonic generation, changes its sign after a few hundred femtoseconds. This is explained by a competition of ballistic and diffusive propagation considering energy-dependent hot carrier relaxation rates. In addition, we observe the decay of the spin polarization within 1 ps, which is associated with the hot carrier spin relaxation time in Au.

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Metadata

Authors
Melnikov, A., Razdolski, I., Wehling, T. O., Papaioannou, E. T., Roddatis, V., Fumagalli, P., Aktsipetrov, O., Lichtenstein, A. I., & Bovensiepen, U.
Venue
Physical Review Letters
Published
2011-08-12
Volume
107
Issue
7
Pages
076601-076601
ISSN
  • 0031-9007 (ISSN-L)
  • 1079-7114
OpenAlex
W2055630667
Cited by
276
References
0
FWCI
7.30
Type
journal article
Language
en
Open access
green

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Melnikov, A., Razdolski, I., Wehling, T. O., Papaioannou, E. T., Roddatis, V., Fumagalli, P., Aktsipetrov, O., Lichtenstein, A. I., & Bovensiepen, U. (2011). Ultrafast Transport of Laser-Excited Spin-Polarized Carriers inAu/Fe/MgO(001). Physical Review Letters. https://doi.org/10.1103/physrevlett.107.076601

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