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Time-Dependent Density Functional Theory for Many-Electron Systems Interacting with Cavity Photons
Open accessAbstract
Time-dependent (current) density functional theory for many-electron systems strongly coupled to quantized electromagnetic modes of a microcavity is proposed. It is shown that the electron-photon wave function is a unique functional of the electronic (current) density and the expectation values of photonic coordinates. The Kohn-Sham system is constructed, which allows us to calculate the above basic variables by solving self-consistent equations for noninteracting particles. We suggest possible approximations for the exchange-correlation potentials and discuss implications of this approach for the theory of open quantum systems. In particular we show that it naturally leads to time-dependent density functional theory for systems coupled to the Caldeira-Leggett bath.
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Cites
Density-Functional Theory for Time-Dependent Systems
Runge, E., & Gross, E. K. U. (1984) · Physical Review Letters · doi:10.1103/physrevlett.52.997 · Cited by 8,914
Strong coupling of a single photon to a superconducting qubit using circuit quantum electrodynamics
Wallraff, A., Schuster, D. I., Blais, A., Frunzio, L., Huang, R. S., Majer, J., Kumar, S., Girvin, S. M., & Schoelkopf, R. J. (2004) · Nature · doi:10.1038/nature02851 · Cited by 3,796
Atomic physics and quantum optics using superconducting circuits
You, J. Q., & Nori, F. (2011) · Nature · doi:10.1038/nature10122 · Cited by 1,311
Cited by
Flick, J., Ruggenthaler, M., Appel, H., & Rubio, A. (2017) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.1615509114 · Cited by 573
Strong light–matter interactions: a new direction within chemistry
Hertzog, M., Wang, M., Mony, J., & Börjesson, K. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00193f · Cited by 444
Polaritonic Chemistry with Organic Molecules
Feist, J., Galego, J., & Garcia-Vidal, F. J. (2018) · ACS Photonics · doi:10.1021/acsphotonics.7b00680 · Cited by 438
Electronic-structure methods for materials design
Marzari, N., Ferretti, A., & Wolverton, C. (2021) · Nature Materials · doi:10.1038/s41563-021-01013-3 · Cited by 253
Metadata
- Authors
- Tokatly, I. V.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2013-06-04
- Volume
- 110
- Issue
- 23
- Pages
- 233001-233001
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2063798031
- Cited by
- 193
- References
- 3
- FWCI
- 2.40
- Type
- journal article
- Language
- en
- Open access
- green
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- Tokatly, I. V. (2013). Time-Dependent Density Functional Theory for Many-Electron Systems Interacting with Cavity Photons. Physical Review Letters. https://doi.org/10.1103/physrevlett.110.233001
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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