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Adsorption Geometry Determination of Single Molecules by Atomic Force Microscopy
Open accessAbstract
We measured the adsorption geometry of single molecules with intramolecular resolution using noncontact atomic force microscopy with functionalized tips. The lateral adsorption position was determined with atomic resolution, adsorption height differences with a precision of 3 pm, and tilts of the molecular plane within 0.2°. The method was applied to five π-conjugated molecules, including three molecules from the olympicene family, adsorbed on Cu(111). For the olympicenes, we found that the substitution of a single atom leads to strong variations of the adsorption height, as predicted by state-of-the-art density-functional theory, including van der Waals interactions with collective substrate response effects.
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Cited by
Unraveling the Molecular Structures of Asphaltenes by Atomic Force Microscopy
Schuler, B., Meyer, G., Peña, D., Mullins, O. C., & Gross, L. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b04056 · Cited by 709
Self-citationAn sp-hybridized molecular carbon allotrope, cyclo[18]carbon
Kaiser, K., Scriven, L. M., Schulz, F., Gawel, P., Gross, L., & Anderson, H. L. (2019) · Science · doi:10.1126/science.aay1914 · Cited by 673
Self-citationA Short History of Cyclocarbons
Anderson, H. L., Patrick, C. W., Scriven, L. M., & Woltering, S. L. (2021) · Bulletin of the Chemical Society of Japan · doi:10.1246/bcsj.20200345 · Cited by 68
Metadata
- Authors
- Schuler, B., Liu, W., Tkatchenko, A., Moll, N., Meyer, G., Mistry, A., Fox, D., & Gross, L.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2013-09-05
- Volume
- 111
- Issue
- 10
- Pages
- 106103-106103
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2088037591
- Cited by
- 194
- References
- 0
- FWCI
- 7.71
- Type
- journal article
- Language
- en
- Open access
- green
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- Schuler, B., Liu, W., Tkatchenko, A., Moll, N., Meyer, G., Mistry, A., Fox, D., & Gross, L. (2013). Adsorption Geometry Determination of Single Molecules by Atomic Force Microscopy. Physical Review Letters. https://doi.org/10.1103/physrevlett.111.106103
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