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Optical Spectrum ofMoS2: Many-Body Effects and Diversity of Exciton States
Open accessAbstract
We present first-principles calculations of the optical response of monolayer molybdenum disulfide employing the GW-Bethe-Salpeter equation (GW-BSE) approach including self-energy, excitonic, and electron-phonon effects. We show that monolayer MoS2 possesses a large and diverse number of strongly bound excitonic states with novel k-space characteristics that were not previously seen experimentally or theoretically. The absorption spectrum is shown to be dominated by excitonic states with a binding energy close to 1 eV and by strong electron-phonon broadening in the visible to ultraviolet range. Our results explain recent experimental measurements and resolve inconsistencies between previous GW-BSE calculations.
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Cited by
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Spin and pseudospins in layered transition metal dichalcogenides
Xu, X., Yao, W., Xiao, D., & Heinz, T. F. (2014) · Nature Physics · doi:10.1038/nphys2942 · Cited by 2,855
Schaibley, J. R., Yu, H., Clark, G., Rivera, P., Ross, J. S., Seyler, K. L., Yao, W., & Xu, X. (2016) · Nature Reviews Materials · doi:10.1038/natrevmats.2016.55 · Cited by 2,652
Jiang, X., Kuklin, A. V., Baev, A., Ge, Y., Ågren, H., Zhang, H., & Prasad, P. N. (2020) · Physics Reports · doi:10.1016/j.physrep.2019.12.006 · Cited by 914
Tunable optical properties of multilayer black phosphorus thin films
Low, T., Rodin, A. S., Carvalho, A., Jiang, Y., Wang, H., Xia, F., & Castro Neto, A. H. (2014) · Physical Review B · doi:10.1103/physrevb.90.075434 · Cited by 722
Metadata
- Authors
- Qiu, D. Y., da Jornada, F. H., & Louie, S. G.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2013-11-20
- Volume
- 111
- Issue
- 21
- Pages
- 216805-216805
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2056902973
- Cited by
- 1,614
- References
- 0
- FWCI
- 50.03
- Type
- journal article
- Language
- en
- Open access
- green
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- Qiu, D. Y., da Jornada, F. H., & Louie, S. G. (2013). Optical Spectrum ofMoS2: Many-Body Effects and Diversity of Exciton States. Physical Review Letters. https://doi.org/10.1103/physrevlett.111.216805
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