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Stimulated Electronic X-Ray Raman Scattering
Open accessAbstract
We demonstrate strong stimulated inelastic x-ray scattering by resonantly exciting a dense gas target of neon with femtosecond, high-intensity x-ray pulses from an x-ray free-electron laser (XFEL). A small number of lower energy XFEL seed photons drive an avalanche of stimulated resonant inelastic x-ray scattering processes that amplify the Raman scattering signal by several orders of magnitude until it reaches saturation. Despite the large overall spectral width, the internal spiky structure of the XFEL spectrum determines the energy resolution of the scattering process in a statistical sense. This is demonstrated by observing a stochastic line shift of the inelastically scattered x-ray radiation. In conjunction with statistical methods, XFELs can be used for stimulated resonant inelastic x-ray scattering, with spectral resolution smaller than the natural width of the core-excited, intermediate state.
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“Despite the ultrahigh intensities necessary for realizing stimulated x-ray emission (10 17 -10 18 W cm -2 in the soft and 10 19 -10 20 W cm -2 in the hard x-ray range), amplified spontaneous x-ray emission [58] and stimulated resonant inelastic x-ray Raman scattering (sRIXS) [59] have been demonstrated in atomic Ne in the soft x-ray spectral range.”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [59]
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Cites
The Theory of Atomic Structure and Spectra
Cowan, R. D. (1981) · University of California Press eBooks · doi:10.1525/9780520906150 · Cited by 5,198
Principles of Nonlinear Optical Spectroscopy
Mukamel, S. (1995) · Cited by 4,640
Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems
Engel, G. S., Calhoun, T. R., Read, E. L., Ahn, T.-K., Mančal, T., Cheng, Y.-C., Blankenship, R. E., & Fleming, G. R. (2007) · Nature · doi:10.1038/nature05678 · Cited by 3,315
First lasing and operation of an ångstrom-wavelength free-electron laser
Emma, P., Akre, R., Arthur, J., Bionta, R., Bostedt, C., Bozek, J., Brachmann, A., Bucksbaum, P., Coffee, R., Decker, F.-J., et al. (2010) · Nature Photonics · doi:10.1038/nphoton.2010.176 · Cited by 3,167
Self-citationA compact X-ray free-electron laser emitting in the sub-ångström region
Ishikawa, T., Aoyagi, H., Asaka, T., Asano, Y., Azumi, N., Bizen, T., Ego, H., Fukami, K., Fukui, T., Furukawa, Y., et al. (2012) · Nature Photonics · doi:10.1038/nphoton.2012.141 · Cited by 1,824
Operation of a free-electron laser from the extreme ultraviolet to the water window
Ackermann, W., Asova, G., Ayvazyan, V., Azima, A., Baboi, N., Bahr, J. W., Balandin, V., Beutner, B., Brandt, A., Bolzmann, A., et al. (2007) · Nature Photonics · doi:10.1038/nphoton.2007.76 · Cited by 1,644
Collective instabilities and high-gain regime in a free electron laser
Bonifacio, R., Pellegrini, C., & Narducci, L. M. (1984) · Optics Communications · doi:10.1016/0030-4018(84)90105-6 · Cited by 1,477
Resonant inelastic x-ray scattering studies of elementary excitations
Ament, L. J. P., van Veenendaal, M., Devereaux, T., Hill, J. P., & van den Brink, J. (2011) · Reviews of Modern Physics · doi:10.1103/revmodphys.83.705 · Cited by 1,289
Structure of the Amide I Band of Peptides Measured by Femtosecond Nonlinear-Infrared Spectroscopy
Hamm, P. M., Lim, M., & Hochstrasser, R. M. (1998) · The Journal of Physical Chemistry B · doi:10.1021/jp9813286 · Cited by 1,095
Resonant inelastic x-ray scattering spectra for electrons in solids
Kotani, A., & Shin, S. (2001) · Reviews of Modern Physics · doi:10.1103/revmodphys.73.203 · Cited by 811
Demonstration of self-seeding in a hard-X-ray free-electron laser
Amann, J., Berg, W. J., Blank, V. D., Decker, F.-J., Ding, Y., Emma, P., Feng, Y., Frisch, J., Fritz, D., Hastings, J. B., et al. (2012) · Nature Photonics · doi:10.1038/nphoton.2012.180 · Cited by 684
Structural Observation of the Primary Isomerization in Vision with Femtosecond-Stimulated Raman
Kukura, P., McCamant, D. W., Yoon, S., Wandschneider, D. B., & Mathies, R. A. (2005) · Science · doi:10.1126/science.1118379 · Cited by 648
Resonant X-ray Raman scattering
Gel’mukhanov, F., & Ågren, H. (1999) · Physics Reports · doi:10.1016/s0370-1573(99)00003-4 · Cited by 481
Simultaneous Femtosecond X-ray Spectroscopy and Diffraction of Photosystem II at Room Temperature
Kern, J. F., Alonso‐Mori, R., Tran, R., Hattne, J., Gildea, R. J., Echols, N., Glöckner, C., Hellmich, J., Laksmono, H., Sierra, R. G., et al. (2013) · Science · doi:10.1126/science.1234273 · Cited by 443
Atomic inner-shell X-ray laser at 1.46 nanometres pumped by an X-ray free-electron laser
Rohringer, N., Ryan, D., London, R. A., Purvis, M., Albert, F., Dunn, J., Bozek, J. D., Bostedt, C., Graf, A., Hill, R., et al. (2012) · Nature · doi:10.1038/nature10721 · Cited by 366
Self-citationCovariance Mapping: A Correlation Method Applied to Multiphoton Multiple Ionization
Frasinski, L. J., Codling, K., & Hatherly, P. A. (1989) · Science · doi:10.1126/science.246.4933.1029 · Cited by 363
Chemical bonding on surfaces probed by X-ray emission spectroscopy and density functional theory
Nilsson, A., & Pettersson, L. G. M. (2004) · Surface Science Reports · doi:10.1016/j.surfrep.2004.06.002 · Cited by 292
Statistical properties of radiation from VUV and X-ray free electron laser
Saldin, E., Schneidmiller, E. A., & Yurkov, M. V. (1998) · Optics Communications · doi:10.1016/s0030-4018(97)00670-6 · Cited by 268
A novel self-seeding scheme for hard X-ray FELs
Geloni, G., Kocharyan, V., & Saldin, E. (2011) · Journal of Modern Optics · doi:10.1080/09500340.2011.586473 · Cited by 261
Experimental Demonstration of Femtosecond Two-Color X-Ray Free-Electron Lasers
Lutman, A. A., Coffee, R., Ding, Y., Huang, Z., Krzywiński, J., Maxwell, T., Messerschmidt, M. M., & Nuhn, H.-D. (2013) · Physical Review Letters · doi:10.1103/physrevlett.110.134801 · Cited by 255
Principles of nonlinear optical spectroscopy
Letokhov, V. S. (1998) · Uspekhi Fizicheskih Nauk · doi:10.3367/ufnr.0168.199805j.0591 · Cited by 202
Mukamel, S., Healion, D., Zhang, Y., & Biggs, J. D. (2013) · Annual Review of Physical Chemistry · doi:10.1146/annurev-physchem-040412-110021 · Cited by 200
Inelastic Resonance Emission of X Rays: Anomalous Scattering Associated with Anomalous Dispersion
Sparks, C. J. (1974) · Physical Review Letters · doi:10.1103/physrevlett.33.262 · Cited by 199
Inelastic x-ray scattering by electronic excitations under high pressure
Rueff, J., & Shukla, A. (2010) · Reviews of Modern Physics · doi:10.1103/revmodphys.82.847 · Cited by 191
Eisenberger, P. M., Platzman, P. M., & Winick, H. (1976) · Physical Review Letters · doi:10.1103/physrevlett.36.623 · Cited by 190
Gain Saturation Regime for Laser-Driven Tabletop, Transient Ni-Like Ion X-Ray Lasers
Dunn, J., Li, Y., Osterheld, A. L., Nilsen, J., Hunter, J., & Shlyaptsev, V. N. (2000) · Physical Review Letters · doi:10.1103/physrevlett.84.4834 · Cited by 176
X-ray nonlinear optical processes using a self-amplified spontaneous emission free-electron laser
Rohringer, N., & Santra, R. (2007) · Physical Review A · doi:10.1103/physreva.76.033416 · Cited by 175
Self-citationThe electronic structure and surface chemistry of glycine adsorbed on Cu(110)
Nyberg, M., Hasselstrøm, J. B., Karis, O., Wassdahl, N., Weinelt, M., Nilsson, A., & Pettersson, L. G. M. (2000) · The Journal of Chemical Physics · doi:10.1063/1.481110 · Cited by 173
Bergmann, U., Glatzel, P., & Cramer, S. P. (2002) · Microchemical Journal · doi:10.1016/s0026-265x(02)00014-0 · Cited by 165
Resonant Inelastic Scattering Spectra of Free Molecules with Vibrational Resolution
Hennies, F., Pietzsch, A., Berglund, M., Föhlisch, A., Schmitt, T., Strocov, V. N., Karlsson, H., Andersson, J., & Rubensson, J. (2010) · Physical Review Letters · doi:10.1103/physrevlett.104.193002 · Cited by 150
Coherent X-Ray Raman Spectroscopy: A Nonlinear Local Probe for Electronic Excitations
Tanaka, S., & Mukamel, S. (2002) · Physical Review Letters · doi:10.1103/physrevlett.89.043001 · Cited by 143
Alonso‐Mori, R., Kern, J. F., Gildea, R. J., Sokaras, D., Weng, T., Lassalle‐Kaiser, B., Tran, R., Hattne, J., Laksmono, H., Hellmich, J., et al. (2012) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.1211384109 · Cited by 139
Stimulated X-ray emission for materials science
Beye, M., Schreck, S., Sorgenfrei, F., Trabant, C., Pontius, N., Schüßler-Langeheine, C., Würth, W., & Föhlisch, A. (2013) · Nature · doi:10.1038/nature12449 · Cited by 124
Sun, Y., Liu, J., Wang, C., & Gel’mukhanov, F. (2010) · Physical Review A · doi:10.1103/physreva.81.013812 · Cited by 70
Maxwell-Bloch modeling of x-ray-laser-signal buildup in single- and double-pass configurations
Larroche, O., Ros, D., Klisnick, A., Sureau, A., Möller, C., & Guennou, H. (2000) · Physical Review A · doi:10.1103/physreva.62.043815 · Cited by 68
FEL-based transient grating spectroscopy to investigate nanoscale dynamics
Bencivenga, F., & Masciovecchio, C. (2009) · Nuclear Instruments and Methods in Physics Research Section A Accelerators Spectrometers Detectors and Associated Equipment · doi:10.1016/j.nima.2009.05.147 · Cited by 51
RIXS investigations of liquids, solutions, and liquid/solid interfaces
Weinhardt, L., Blum, M., Fuchs, O., Benkert, A., Meyer, F., Bär, M., Denlinger, J. D., Yang, W., Reinert, F., & Heske, C. (2012) · Journal of Electron Spectroscopy and Related Phenomena · doi:10.1016/j.elspec.2012.10.006 · Cited by 47
Amplified X-Ray Emission from Core-Ionized Diatomic Molecules
Kimberg, V., & Rohringer, N. (2013) · Physical Review Letters · doi:10.1103/physrevlett.110.043901 · Cited by 43
Self-citationTwo-bunch self-seeding for narrow-bandwidth hard x-ray free-electron lasers
Ding, Y., Huang, Z., & Ruth, R. D. (2010) · Physical Review Special Topics - Accelerators and Beams · doi:10.1103/physrevstab.13.060703 · Cited by 36
Harbola, U., & Mukamel, S. (2009) · Physical Review B · doi:10.1103/physrevb.79.085108 · Cited by 36
Strongly driven resonant Auger effect treated by an open-quantum-system approach
Rohringer, N., & Santra, R. (2012) · Physical Review A · doi:10.1103/physreva.86.043434 · Cited by 34
Self-citationStimulated resonant x-ray Raman scattering with incoherent radiation
Weninger, C., & Rohringer, N. (2013) · Physical Review A · doi:10.1103/physreva.88.053421 · Cited by 33
Self-citationHealion, D., Wang, H., & Mukamel, S. (2011) · The Journal of Chemical Physics · doi:10.1063/1.3557057 · Cited by 25
Pulse buildup from noise and intrinsic polarization of plasma-based x-ray lasers
Kim, C. M., Janulewicz, K. A., & Lee, J. (2011) · Physical Review A · doi:10.1103/physreva.84.013834 · Cited by 15
Miao, Q., Liu, J., Ågren, H., Rubensson, J., & Gel’mukhanov, F. (2012) · Physical Review Letters · doi:10.1103/physrevlett.109.233905 · Cited by 15
Oura, M. (2010) · Plasma Science and Technology · doi:10.1088/1009-0630/12/3/21 · Cited by 12
Stimulated Raman scattering in helium with soft-x-ray laser radiation
Fill, E. E., van Enk, S. J., Zhang, J., & Lambropoulos, P. (1996) · Physical Review A · doi:10.1103/physreva.54.5374 · Cited by 11
X-ray lasing in the CO molecule
Kimberg, V., Zhang, S. B., & Rohringer, N. (2013) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/0953-4075/46/16/164017 · Cited by 10
Self-citationX-ray-stimulated electronic Raman scattering in neutral gases and inhibited ionization
Hudis, E., Shkolnikov, P. L., & Kaplan, A. E. (1994) · Journal of the Optical Society of America B · doi:10.1364/josab.11.001158 · Cited by 9
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Metadata
- Authors
- Weninger, C., Purvis, M., Ryan, D., London, R. A., Bozek, J. D., Bostedt, C., Graf, A., Brown, G., Rocca, J. J., & Rohringer, N.
- Affiliations
- Max Planck Institute for the Physics of Complex Systems (DE)
- Colorado State University (US)
- Lawrence Livermore National Laboratory (US)
- SLAC National Accelerator Laboratory (US)
- ORCID
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2013-12-05
- Volume
- 111
- Issue
- 23
- Pages
- 233902-233902
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2032189197
- Cited by
- 148
- References
- 49
- Citations by year
- 2026: 4 · 2025: 9 · 2024: 13 · 2023: 12 · 2022: 9 · 2021: 16 · 2020: 14 · 2019: 14 · 2018: 9 · 2017: 3 · 2016: 13 · 2015: 23 · 2014: 9
- FWCI
- 7.72
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Locations
- Physical Review Letters (publishedVersion)
- PubMed (publishedVersion)
- DESY Publication Database (PUBDB) (Deutsches Elektronen-Synchrotron) (submittedVersion, other-oa)
- Max Planck Institute for Plasma Physics (submittedVersion)
- Max Planck Digital Library (submittedVersion, other-oa)
- MPG.PuRe (Max Planck Society) (submittedVersion)
- Funders
- U.S. Department of Energy (DEAC5207NA27344, AC52‐07NA27344, Contract No. DE-AC52-07NA27344, No. DE-AC52-07NA27344)
- Office of Science (DE-AC52-07NA27344)
- Basic Energy Sciences (DE-AC52-07NA27344.)
- Lawrence Livermore National Laboratory (DE‐AC5207NA27344, No. DE-AC52-07NA27344, AC52-07NA27344)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Radiation › X-ray Spectroscopy and Fluorescence Analysis
- Physical Sciences › Physics and Astronomy › Radiation › Advanced X-ray Imaging Techniques
- Keywords
- stimulated Raman scattering, X-ray free-electron laser, neon gas, femtosecond X-ray pulses, signal amplification, spectral resolution, core-excited states, intermediate state, line shift, statistical analysis
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