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Electronic Structure of the Silicon Vacancy Color Center in Diamond

Open access
Hepp, Christian, Müller, Tina, Waselowski, Victor, Becker, Jonas N., Pingault, Benjamin, Sternschulte, Hadwig, Steinmüller-Nethl, Doris, Gali, Adam, Maze, Jeronimo R., Atatüre, Mete, Becher, Christoph·2014·Physical Review Letters

Abstract

The negatively charged silicon vacancy (SiV) color center in diamond has recently proven its suitability for bright and stable single photon emission. However, its electronic structure so far has remained elusive. We here explore the electronic structure by exposing single SiV defects to a magnetic field where the Zeeman effect lifts the degeneracy of magnetic sublevels. The similar responses of single centers and a SiV ensemble in a low strain reference sample prove our ability to fabricate almost perfect single SiVs, revealing the true nature of the defect's electronic properties. We model the electronic states using a group-theoretical approach yielding a good agreement with the experimental observations. Furthermore, the model correctly predicts polarization measurements on single SiV centers and explains recently discovered spin selective excitation of SiV defects.

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Metadata

Authors
Hepp, C., Müller, T., Waselowski, V., Becker, J. N., Pingault, B., Sternschulte, H., Steinmüller-Nethl, D., Gali, A., Maze, J. R., Atatüre, M., & Becher, C.
Venue
Physical Review Letters
Published
2014-01-24
Volume
112
Issue
3
Pages
036405-036405
ISSN
  • 0031-9007 (ISSN-L)
  • 1079-7114
OpenAlex
W2115456012
Cited by
432
References
0
FWCI
12.81
Type
journal article
Language
en
Open access
green

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CoChat. (2026). Citation check: Electronic Structure of the Silicon Vacancy Color Center in Diamond. https://app.cochat.ai/papers/10.1103/physrevlett.112.036405
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Hepp, C., Müller, T., Waselowski, V., Becker, J. N., Pingault, B., Sternschulte, H., Steinmüller-Nethl, D., Gali, A., Maze, J. R., Atatüre, M., & Becher, C. (2014). Electronic Structure of the Silicon Vacancy Color Center in Diamond. Physical Review Letters. https://doi.org/10.1103/physrevlett.112.036405

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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).

Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.