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Spatial Coherence Properties of Organic Molecules Coupled to Plasmonic Surface Lattice Resonances in the Weak and Strong Coupling Regimes
Open accessAbstract
We study spatial coherence properties of a system composed of periodic silver nanoparticle arrays covered with a fluorescent organic molecule (DiD) film. The evolution of spatial coherence of this composite structure from the weak to the strong coupling regime is investigated by systematically varying the coupling strength between the localized DiD excitons and the collective, delocalized modes of the nanoparticle array known as surface lattice resonances. A gradual evolution of coherence from the weak to the strong coupling regime is observed, with the strong coupling features clearly visible in interference fringes. A high degree of spatial coherence is demonstrated in the strong coupling regime, even when the mode is very excitonlike (80%), in contrast to the purely localized nature of molecular excitons. We show that coherence appears in proportion to the weight of the plasmonic component of the mode throughout the weak-to-strong coupling crossover, providing evidence for the hybrid nature of the normal modes.
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Cites
Spontaneous Coherent Phase Transition of Polaritons in CdTe Microcavities
Richard, M., Kasprzak, J., Romestain, R., André, R., & Dang, L. S. (2005) · Physical Review Letters · doi:10.1103/physrevlett.94.187401 · Cited by 173
Cited by
Strong coupling between surface plasmon polaritons and emitters: a review
Törmä, P., & Barnes, W. L. (2015) · Reports on Progress in Physics · doi:10.1088/0034-4885/78/1/013901 · Cited by 1,644
Self-citationConductivity in organic semiconductors hybridized with the vacuum field
Orgiu, E., George, J., Hutchison, J. A., Devaux, E., Dayen, J. F., Doudin, B., Stellacci, F., Genet, C., Schachenmayer, J., Genes, C., et al. (2015) · Nature Materials · doi:10.1038/nmat4392 · Cited by 615
Novel Nanostructures and Materials for Strong Light–Matter Interactions
Baranov, D. G., Wersäll, M., Cuadra, J., Antosiewicz, T. J., & Shegai, T. (2018) · ACS Photonics · doi:10.1021/acsphotonics.7b00674 · Cited by 531
Strong light–matter interactions: a new direction within chemistry
Hertzog, M., Wang, M., Mony, J., & Börjesson, K. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00193f · Cited by 444
Strong Light-Matter Interactions in Single Open Plasmonic Nanocavities at the Quantum Optics Limit
Liu, R., Zhou, Z.-K., Yu, Y.-C., Zhang, T., Wang, H., Liu, G., Wei, Y., Chen, H., & Wang, X.-H. (2017) · Physical Review Letters · doi:10.1103/physrevlett.118.237401 · Cited by 293
Metadata
- Authors
- Shi, L., Hakala, T. K., Rekola, H. T., Martikainen, J.-P., Moerland, R. J., & Törmä, P.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2014-04-14
- Volume
- 112
- Issue
- 15
- Pages
- 153002-153002
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2067747909
- Cited by
- 195
- References
- 1
- FWCI
- 10.93
- Type
- journal article
- Language
- en
- Open access
- green
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- Shi, L., Hakala, T. K., Rekola, H. T., Martikainen, J.-P., Moerland, R. J., & Törmä, P. (2014). Spatial Coherence Properties of Organic Molecules Coupled to Plasmonic Surface Lattice Resonances in the Weak and Strong Coupling Regimes. Physical Review Letters. https://doi.org/10.1103/physrevlett.112.153002
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