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Hund’s Rule-Driven Dzyaloshinskii-Moriya Interaction at3d−5dInterfaces
Open accessAbstract
Using relativistic first-principles calculations, we show that the chemical trend of the Dzyaloshinskii-Moriya interaction (DMI) in 3d-5d ultrathin films follows Hund's first rule with a tendency similar to their magnetic moments in either the unsupported 3d monolayers or 3d-5d interfaces. We demonstrate that, besides the spin-orbit coupling (SOC) effect in inversion asymmetric noncollinear magnetic systems, the driving force is the 3d orbital occupations and their spin-flip mixing processes with the spin-orbit active 5d states control directly the sign and magnitude of the DMI. The magnetic chirality changes are discussed in the light of the interplay between SOC, Hund's first rule, and the crystal-field splitting of d orbitals.
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Citations
Cites
Self-interaction correction to density-functional approximations for many-electron systems
Perdew, J. P., & Zunger, A. (1981) · Physical Review B · doi:10.1103/physrevb.23.5048 · Cited by 20,887
Anisotropic Superexchange Interaction and Weak Ferromagnetism
Moriya, T. (1960) · Physical Review · doi:10.1103/physrev.120.91 · Cited by 7,234
Cited by
Tokura, Y., & Kanazawa, N. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00297 · Cited by 726
Skyrmions in magnetic multilayers
Jiang, W., Chen, G., Liu, K., Zang, J., te Velthuis, S. G. E., & Hoffmann, A. (2017) · Physics Reports · doi:10.1016/j.physrep.2017.08.001 · Cited by 566
First-principles calculations for Dzyaloshinskii–Moriya interaction
Yang, H., Liang, J., & Cui, Q. (2022) · Nature Reviews Physics · doi:10.1038/s42254-022-00529-0 · Cited by 194
Metadata
- Authors
- Belabbes, A., Bihlmayer, G., Bechstedt, F., Blügel, S., & Manchon, A.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2016-12-09
- Volume
- 117
- Issue
- 24
- Pages
- 247202-247202
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2520815513
- Cited by
- 218
- References
- 2
- FWCI
- 8.26
- Type
- journal article
- Language
- en
- Open access
- green
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- Belabbes, A., Bihlmayer, G., Bechstedt, F., Blügel, S., & Manchon, A. (2016). Hund’s Rule-Driven Dzyaloshinskii-Moriya Interaction at3d−5dInterfaces. Physical Review Letters. https://doi.org/10.1103/physrevlett.117.247202
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