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Defect Structure of Localized Excitons in a WSe2 Monolayer
Abstract
The atomic and electronic structure of intrinsic defects in a WSe_{2} monolayer grown on graphite was revealed by low temperature scanning tunneling microscopy and spectroscopy. Instead of chalcogen vacancies that prevail in other transition metal dichalcogenide materials, intrinsic defects in WSe_{2} arise surprisingly from single tungsten vacancies, leading to the hole (p-type) doping. Furthermore, we found these defects to dominate the excitonic emission of the WSe_{2} monolayer at low temperature. Our work provided the first atomic-scale understanding of defect excitons and paved the way toward deciphering the defect structure of single quantum emitters previously discovered in the WSe_{2} monolayer.
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Cites
Spin and pseudospins in layered transition metal dichalcogenides
Xu, X., Yao, W., Xiao, D., & Heinz, T. F. (2014) · Nature Physics · doi:10.1038/nphys2942 · Cited by 2,855
Schaibley, J. R., Yu, H., Clark, G., Rivera, P., Ross, J. S., Seyler, K. L., Yao, W., & Xu, X. (2016) · Nature Reviews Materials · doi:10.1038/natrevmats.2016.55 · Cited by 2,652
Solid-state single-photon emitters
Aharonovich, I., Englund, D., & Toth, M. (2016) · Nature Photonics · doi:10.1038/nphoton.2016.186 · Cited by 1,786
Cited by
Disorder in van der Waals heterostructures of 2D materials
Rhodes, D., Chae, S. H., Ribeiro-Palau, R., & Hone, J. (2019) · Nature Materials · doi:10.1038/s41563-019-0366-8 · Cited by 656
Atomically thin quantum light-emitting diodes
Palacios-Berraquero, C., Barbone, M., Kara, D. M., Chen, X., Goykhman, I., Yoon, D., Ott, A. K., Beitner, J., Watanabe, K., Taniguchi, T., et al. (2016) · Nature Communications · doi:10.1038/ncomms12978 · Cited by 334
Quantum photonics with layered 2D materials
Turunen, M., Brotons-Gisbert, M., Dai, Y., Wang, Y., Scerri, E., Bonato, C., Jöns, K. D., Sun, Z., & Gerardot, B. D. (2022) · Nature Reviews Physics · doi:10.1038/s42254-021-00408-0 · Cited by 259
Metadata
- Authors
- Zhang, S., Wang, C.-G., Li, M.-Y., Huang, D., Li, L.-J., Ji, W., & Wu, S.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2017-07-25
- Volume
- 119
- Issue
- 4
- Pages
- 046101-046101
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2737675653
- Cited by
- 237
- References
- 3
- FWCI
- 9.94
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, S., Wang, C.-G., Li, M.-Y., Huang, D., Li, L.-J., Ji, W., & Wu, S. (2017). Defect Structure of Localized Excitons in a WSe2 Monolayer. Physical Review Letters. https://doi.org/10.1103/physrevlett.119.046101
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