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Observation of Rotational Excitations ofH2Adsorbed on Ag Surfaces
Abstract
High-resolution electron-energy-loss studies of ${\mathrm{H}}_{2}$ on Ag at \ensuremath{\sim} 10 K reveal both rotational and rotational-vibrational excitations of molecularly adsorbed and condensed ${\mathrm{H}}_{2}$. The rotational losses for submonolayers of adsorbed ${\mathrm{H}}_{2}$ indicate unhindered rotational motion as well as a H-H internuclear separation which is within \ensuremath{\sim}2% of that of condensed ${\mathrm{H}}_{2}$. Adsorbed ${\mathrm{H}}_{2}$ is also converted from predominantly orthohydrogen to parahydrogen.
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“Some materials, such as silver [81][82][83], copper [84,85], charcoal [56], graphite [86], and supported chromium [87,88] and ferric [89,90] oxides, have been found to be effective for this conversion.”
From 5917. https://doi.org/10.3390/en14185917. - (2021) · cites this paper as [81]
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“Some materials, such as silver[81][82][83], copper[84,85], charcoal[56], graphite[86], and supported chromium[87,88] and ferric[89,90] oxides, have been found to be effective for this conversion.”
From 5917. https://doi.org/10.3390/en14185917. - (2021) · cites this paper as [81]
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(2021) · doi:10.3390/en14185917 · Cited by 708
Metadata
- Authors
- Avouris, P., Schmeisser, D., & Demuth, J. E.
- Affiliations
- IBM Research - Thomas J. Watson Research Center (US)
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 1982-01-18
- Volume
- 48
- Issue
- 3
- Pages
- 199-202
- ISSN
- 0031-9007 (ISSN-L)
- OpenAlex
- W2058296579
- Cited by
- 181
- References
- 0
- Citations by year
- 2026: 1 · 2025: 2 · 2024: 1 · 2023: 2 · 2022: 1 · 2021: 3 · 2020: 3 · 2019: 2 · 2018: 2 · 2017: 1 · 2016: 5 · 2015: 4 · 2014: 4 · 2013: 8 · 2012: 3
- FWCI
- 12.89
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Physical Review Letters (publishedVersion)
- Topics
- Physical Sciences › Chemistry › Physical and Theoretical Chemistry › Surface Chemistry and Catalysis
- Physical Sciences › Materials Science › Surfaces, Coatings and Films › Electron and X-Ray Spectroscopy Techniques
- Physical Sciences › Physics and Astronomy › Condensed Matter Physics › Surface and Thin Film Phenomena
- Keywords
- molecular hydrogen adsorption, silver surface, rotational excitation, electron energy loss spectroscopy, submonolayer adsorption, hydrogen condensation, low-temperature adsorption
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