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Critical Behavior of Binary Liquid Mixtures of Deuterated and Protonated Polymers
Abstract
Binary mixtures of protonated and perdeuterated 1,4-polybutadiene have been examined by small-angle neutron scattering and are shown to exhibit an upper critical solution temperature. The scattering results above the critical temperature are described by the mean-field theory of de Gennes for homogeneous binary polymer mixtures. These results contradict the universally held assumption that mixtures of deuterated and protonated polymers of otherwise identical chemical structure form ideal solutions.
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Citations
Cited by
Polymer-polymer phase behavior
Bates, F. S. (1991) · Science · doi:10.1126/science.251.4996.898 · Cited by 1,463
Self-citationSpinodal decomposition of a symmetric critical mixture of deuterated and protonated polymer
Bates, F. S., & Wiltzius, P. (1989) · The Journal of Chemical Physics · doi:10.1063/1.456901 · Cited by 388
Self-citationIntegral Equation Theories of the Structure, Thermodynamics, and Phase Transitions of Polymer Fluids
Schweizer, K. S., & Curro, J. G. (1997) · Advances in Chemical Physics · doi:10.1002/9780470141571.ch1 · Cited by 386
Surface Enrichment in an Isotopic Polymer Blend
Jones, R. A. L., Kramer, E. J., Rafailovich, M. H., Sokolov, J., & Schwarz, S. A. (1989) · Physical Review Letters · doi:10.1103/physrevlett.62.280 · Cited by 269
Krishnaswamy, R. K., & Yang, Q. (2007) · Polymer · doi:10.1016/j.polymer.2007.07.018 · Cited by 16
Metadata
- Authors
- Bates, F. S., Wignall, G. D., & Koehler, W. C.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 1985-11-25
- Volume
- 55
- Issue
- 22
- Pages
- 2425-2428
- ISSN
- 0031-9007 (ISSN-L)
- OpenAlex
- W1969262298
- Cited by
- 222
- References
- 0
- FWCI
- 11.15
- Type
- journal article
- Language
- en
- Open access
- closed
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- Bates, F. S., Wignall, G. D., & Koehler, W. C. (1985). Critical Behavior of Binary Liquid Mixtures of Deuterated and Protonated Polymers. Physical Review Letters. https://doi.org/10.1103/physrevlett.55.2425
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
