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Sum-frequency vibrational spectroscopy of a Langmuir film: Study of molecular orientation of a two-dimensional system
Abstract
Using infrared-visible sum-frequency generation as a probe, we have obtained the vibrational spectrum of a monolayer of pentadecanoic acid on a water surface in the CH stretch region. We have monitored the molecular orientation at different surface densities. It was found that the molecules in the liquid condensed phase have their alkane chains extended and oriented nearly normal to the surface, while in the liquid expanded phase the chains are highly disordered.
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Citations
Cited by
Coherent Two-Dimensional Optical Spectroscopy
Cho, M. (2008) · Chemical Reviews · doi:10.1021/cr078377b · Cited by 835
Interfacial water dielectric-permittivity-profile measurements using atomic force microscopy
Teschke, O., Ceotto, G., & de Souza, E. F. (2001) · Physical Review E · doi:10.1103/physreve.64.011605 · Cited by 209
Metadata
- Authors
- Guyot-Sionnest, P., Hunt, J. H., & Shen, Y. R.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 1987-10-05
- Volume
- 59
- Issue
- 14
- Pages
- 1597-1600
- ISSN
- 0031-9007 (ISSN-L)
- OpenAlex
- W2085161139
- Cited by
- 670
- References
- 0
- FWCI
- 8.87
- Type
- journal article
- Language
- en
- Open access
- closed
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- Guyot-Sionnest, P., Hunt, J. H., & Shen, Y. R. (1987). Sum-frequency vibrational spectroscopy of a Langmuir film: Study of molecular orientation of a two-dimensional system. Physical Review Letters. https://doi.org/10.1103/physrevlett.59.1597
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
