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New spectroscopy of water using tunable picosecond pulses in the infrared
Abstract
Spectral hole burning is observed for the OH stretching mode of HDO dissolved in ${\mathrm{D}}_{2}$O at 298 K after intense infrared excitation. Three spectral components are inferred from the transient band shapes and related to an icelike molecular environment and other hydrogen-bonding configurations. A population lifetime of ${\mathit{T}}_{1}$=8\ifmmode\pm\else\textpm\fi{}2 ps and an anharmonic frequency shift of 270\ifmmode\pm\else\textpm\fi{}20 ${\mathrm{cm}}^{\mathrm{\ensuremath{-}}1}$ are measured.
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Citations
Cited by
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Müller-Dethlefs, K., & Hobza, P. (2000) · Chemical Reviews · doi:10.1021/cr9900331 · Cited by 1,781
Coherent Two-Dimensional Optical Spectroscopy
Cho, M. (2008) · Chemical Reviews · doi:10.1021/cr078377b · Cited by 835
Metadata
- Authors
- Graener, H., Seifert, G., & Laubereau, A.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 1991-04-22
- Volume
- 66
- Issue
- 16
- Pages
- 2092-2095
- ISSN
- 0031-9007 (ISSN-L)
- OpenAlex
- W2011478408
- Cited by
- 217
- References
- 0
- FWCI
- 3.88
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: New spectroscopy of water using tunable picosecond pulses in the infrared. https://app.cochat.ai/papers/10.1103/physrevlett.66.2092
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- Graener, H., Seifert, G., & Laubereau, A. (1991). New spectroscopy of water using tunable picosecond pulses in the infrared. Physical Review Letters. https://doi.org/10.1103/physrevlett.66.2092
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
