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Epitaxial Relationship for Hexagonal-to-Cubic Phase Transition in a Book Copolymer Mixture
Abstract
Small-angle neutron scattering experiments have revealed an epitaxial relationship between the hexagonal cylinder phase, and a bicontinuous cubic phase with $\mathrm{Ia}\overline{3}d$ space group symmetry, in a poly(styrene)-poly(2-vinylpyridine) diblock copolymer mixture. Proximity to the order-disorder transition and an inelastic low frequency rheological response suggest that the cubic phase is stabilized by fluctuations. These results identify block copolymers as model compounds for investigating the thermodynamics and dynamics of complex "soft" condensed matter.
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Citations
Cited by
Block Copolymers—Designer Soft Materials
Bates, F. S., & Fredrickson, G. H. (1999) · Physics Today · doi:10.1063/1.882522 · Cited by 3,219
Self-citation50th Anniversary Perspective: Block Polymers—Pure Potential
Bates, C. M., & Bates, F. S. (2017) · Macromolecules · doi:10.1021/acs.macromol.6b02355 · Cited by 788
Self-citationHan, L., & Che, S. (2018) · Advanced Materials · doi:10.1002/adma.201705708 · Cited by 624
Origins of complex self-assembly in block copolymers
Matsen, M. W., & Bates, F. S. (1996) · Macromolecules · doi:10.1021/ma960744q · Cited by 578
Self-citationPhase Behaviour and Morphologies of Block Copolymers
Abetz, V., & Simon, P. F. W. (2005) · Advances in Polymer Science · doi:10.1007/12_004 · Cited by 361
Metadata
- Authors
- Schulz, M. F., Bates, F. S., Almdal, K., & Mortensen, K.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 1994-07-04
- Volume
- 73
- Issue
- 1
- Pages
- 86-89
- ISSN
- 0031-9007 (ISSN-L)
- OpenAlex
- W1969817290
- Cited by
- 273
- References
- 0
- FWCI
- 9.74
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Epitaxial Relationship for Hexagonal-to-Cubic Phase Transition in a Book Copolymer Mixture. https://app.cochat.ai/papers/10.1103/physrevlett.73.86
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- Schulz, M. F., Bates, F. S., Almdal, K., & Mortensen, K. (1994). Epitaxial Relationship for Hexagonal-to-Cubic Phase Transition in a Book Copolymer Mixture. Physical Review Letters. https://doi.org/10.1103/physrevlett.73.86
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
