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Experimental Determination of the Quantum-Mechanical State of a Molecular Vibrational Mode Using Fluorescence Tomography
Abstract
We present a spectroscopic method for the complete characterization of the quantum state of the vibrational mode of a molecule in terms of a phase-space quasiprobability distribution. The distribution for a molecular vibrational mode excited by a short optical pulse is reconstructed from measurements of its time-dependent spectrum of fluorescence.
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Smithey, D. T., Beck, M., Raymer, M. G., & Faridani, A. (1993) · Physical Review Letters · doi:10.1103/physrevlett.70.1244 · Cited by 1,538
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Leibfried, D., Blatt, R., Monroe, C., & Wineland, D. (2003) · Reviews of Modern Physics · doi:10.1103/revmodphys.75.281 · Cited by 2,739
Tomographic imaging of molecular orbitals
Itatani, J., Levesque, J., Zeidler, D., Niikura, H., Pépin, H., Kieffer, J. C., Corkum, P. B., & Villeneuve, D. M. (2004) · Nature · doi:10.1038/nature03183 · Cited by 2,309
James, D. F. V., Kwiat, P. G., Munro, W. J., & White, A. G. (2001) · Physical Review A · doi:10.1103/physreva.64.052312 · Cited by 2,176
Quantum computing with trapped ions
HAFFNER, H., ROOS, C., & BLATT, R. (2008) · Physics Reports · doi:10.1016/j.physrep.2008.09.003 · Cited by 1,154
Continuous-variable optical quantum-state tomography
Lvovsky, A. I., & Raymer, M. G. (2009) · Reviews of Modern Physics · doi:10.1103/revmodphys.81.299 · Cited by 1,123
Metadata
- Authors
- Dunn, T. J., Walmsley, I. A., & Mukamel, S.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 1995-02-06
- Volume
- 74
- Issue
- 6
- Pages
- 884-887
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2061054805
- Cited by
- 324
- References
- 1
- FWCI
- 20.01
- Type
- journal article
- Language
- en
- Open access
- closed
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- Dunn, T. J., Walmsley, I. A., & Mukamel, S. (1995). Experimental Determination of the Quantum-Mechanical State of a Molecular Vibrational Mode Using Fluorescence Tomography. Physical Review Letters. https://doi.org/10.1103/physrevlett.74.884
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.