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Zeolite-Dye Microlasers
Open accessAbstract
We present a new class of micro lasers based on nanoporous molecular sieve host-guest systems. Organic dye guest molecules of 1-ethyl-4-[4-( $p$-dimethylaminophenyl)-1,3-butadienyl]-pyridinium Perchlorat were inserted into the 0.73-nm-wide channel pores of a zeolite $\mathrm{AlPO}{}_{4}\ensuremath{-}5$ host. The zeolitic microcrystal compounds were hydrothermally synthesized according to a particular host-guest chemical process. The dye molecules are found not only to be aligned along the host channel axis, but to be oriented as well. Single mode laser emission at $687\mathrm{nm}$ was obtained from a whispering gallery mode oscillating in a $8\ensuremath{-}\ensuremath{\mu}\mathrm{m}\ensuremath{-}\mathrm{diameter}$ monolithic microresonator, in which the field is confined by total internal reflection at the natural hexagonal boundaries inside the zeolitic microcrystals.
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Citations
Cited by
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Davis, M. E. (2002) · Nature · doi:10.1038/nature00785 · Cited by 5,308
Dielectric microcavities: Model systems for wave chaos and non-Hermitian physics
Cao, H., & Wiersig, J. (2015) · Reviews of Modern Physics · doi:10.1103/revmodphys.87.61 · Cited by 686
Mirrorless Lasing from Mesostructured Waveguides Patterned by Soft Lithography
Yang, P., Wirnsberger, †. G., Huang, H. C., Cordero, S. R., McGehee, M. D., Scott, B., Deng, T., Whitesides, G. M., Chmelka, B. F., Buratto, S. K., et al. (2000) · Science · doi:10.1126/science.287.5452.465 · Cited by 478
Whispering Gallery Modes in Nanosized Dielectric Resonators with Hexagonal Cross Section
Nobis, T., Kaidashev, E. M., Rahm, A., Lorenz, M., & Grundmann, M. (2004) · Physical Review Letters · doi:10.1103/physrevlett.93.103903 · Cited by 305
Kahr, B., & Gurney, R. W. (2001) · Chemical Reviews · doi:10.1021/cr980088n · Cited by 299
Metadata
- Authors
- Vietze, U., Krauß, O., Laeri, F., Ihlein, G., Schüth, F., Limburg, B., & Abraham, M.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 1998-11-23
- Volume
- 81
- Issue
- 21
- Pages
- 4628-4631
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2018419636
- Cited by
- 180
- References
- 0
- FWCI
- 6.42
- Type
- journal article
- Language
- en
- Open access
- green
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- Vietze, U., Krauß, O., Laeri, F., Ihlein, G., Schüth, F., Limburg, B., & Abraham, M. (1998). Zeolite-Dye Microlasers. Physical Review Letters. https://doi.org/10.1103/physrevlett.81.4628
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