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Resonant and Off-Resonant Light-Driven Plasmons in Metal Nanoparticles Studied by Femtosecond-Resolution Third-Harmonic Generation
Abstract
We report on a femtosecond-resolution study of the plasmon fields in gold nanoparticles using third-harmonic generation. Controlled resonant and off-resonant plasmon excitation is achieved by tailoring the nanoparticle sample by an electron-beam-lithographic method. Comparing the measured third order interferometric autocorrelation function of the plasmon field with simulations based on a simple harmonic oscillator model we extract the temporal characteristic of the plasmon oscillation. For off-resonant excitation of particle plasmons we find a beating between the driving laser field and the plasmon field which demonstrates clearly the nature of the plasmon as a collective electron oscillation.
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Citations
Cited by
Plasmonics: Localization and guiding of electromagnetic energy in metal/dielectric structures
Maier, S. A., & Atwater, H. A. (2005) · Journal of Applied Physics · doi:10.1063/1.1951057 · Cited by 1,923
Metal Nanoparticle Gratings: Influence of Dipolar Particle Interaction on the Plasmon Resonance
Lamprecht, B., Schider, G., Lechner, R. T., Ditlbacher, H., Krenn, J. R., Leitner, A., & Aussenegg, F. R. (2000) · Physical Review Letters · doi:10.1103/physrevlett.84.4721 · Cited by 586
Self-citationQuantum hydrodynamic model for the nonlinear electron dynamics in thin metal films
Crouseilles, N., Hervieux, P.-A., & Manfredi, G. (2008) · Physical Review B · doi:10.1103/physrevb.78.155412 · Cited by 346
Hanke, T., Krauss, G., Träutlein, D., Wild, B., Bratschitsch, R., & Leitenstorfer, A. (2009) · Physical Review Letters · doi:10.1103/physrevlett.103.257404 · Cited by 261
Phase-space modeling of solid-state plasmas: A journey from classical to quantum
Manfredi, G., Hervieux, P.-A., & Hurst, J. (2019) · Reviews of Modern Plasma Physics · doi:10.1007/s41614-019-0034-0 · Cited by 38
Metadata
- Authors
- Lamprecht, B., Krenn, J. R., Leitner, A., & Aussenegg, F. R.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 1999-11-22
- Volume
- 83
- Issue
- 21
- Pages
- 4421-4424
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2011085460
- Cited by
- 208
- References
- 0
- FWCI
- 7.71
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Resonant and Off-Resonant Light-Driven Plasmons in Metal Nanoparticles Studied by Femtosecond-Resolution Third-Harmonic Generation. https://app.cochat.ai/papers/10.1103/physrevlett.83.4421
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- Lamprecht, B., Krenn, J. R., Leitner, A., & Aussenegg, F. R. (1999). Resonant and Off-Resonant Light-Driven Plasmons in Metal Nanoparticles Studied by Femtosecond-Resolution Third-Harmonic Generation. Physical Review Letters. https://doi.org/10.1103/physrevlett.83.4421
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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