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Time-Resolved X-Ray Diffraction from Coherent Phonons during a Laser-Induced Phase Transition
Open accessAbstract
Time-resolved x-ray diffraction with picosecond temporal resolution is used to observe scattering from impulsively generated coherent acoustic phonons in laser-excited InSb crystals. The observed frequencies and damping rates are in agreement with a model based on dynamical diffraction theory coupled to analytic solutions for the laser-induced strain profile. The results are consistent with a 12 ps thermal electron-acoustic phonon coupling time together with an instantaneous component from the deformation-potential interaction. Above a critical laser fluence, we show that the first step in the transition to a disordered state is the excitation of large amplitude, coherent atomic motion.
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Cited by
Non-thermal melting in semiconductors measured at femtosecond resolution
Rousse, A., Rischel, C., Fourmaux, S., Uschmann, I., Sebban, S., Grillon, G., Balcou, P., Förster, E., Geindre, J. P., Audebert, P., et al. (2001) · Nature · doi:10.1038/35065045 · Cited by 729
Femtosecond X-ray measurement of coherent lattice vibrations near the Lindemann stability limit
Sokolowski-Tinten, K., Blome, C., Blums, J., Cavalleri, A., Dietrich, C., Tarasevitch, A., Uschmann, I., Förster, E., Kammler, M., Horn-von-Hoegen, M., et al. (2003) · Nature · doi:10.1038/nature01490 · Cited by 639
Ultrafast X-ray Absorption Spectroscopy
Bressler, C., & Chergui, M. (2004) · Chemical Reviews · doi:10.1021/cr0206667 · Cited by 493
Femtosecond electron diffraction: heralding the era of atomically resolved dynamics
Sciaini, G., & Miller, R. J. D. (2011) · Reports on Progress in Physics · doi:10.1088/0034-4885/74/9/096101 · Cited by 485
Giannetti, C., Capone, M., Fausti, D., Fabrizio, M., Parmigiani, F., & Mihailovic, D. (2016) · Advances in Physics · doi:10.1080/00018732.2016.1194044 · Cited by 481
Metadata
- Authors
- Lindenberg, A. M., Kang, I., Johnson, S. L., Missalla, T., Heimann, P. A., Chang, Z., Larsson, J., Bucksbaum, P. H., Kapteyn, H. C., Padmore, H. A., Lee, R. W., Wark, J. S., & Falcone, R. W.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2000-01-03
- Volume
- 84
- Issue
- 1
- Pages
- 111-114
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W1982806915
- Cited by
- 373
- References
- 0
- FWCI
- 20.39
- Type
- journal article
- Language
- en
- Open access
- bronze
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- The paper
- Lindenberg, A. M., Kang, I., Johnson, S. L., Missalla, T., Heimann, P. A., Chang, Z., Larsson, J., Bucksbaum, P. H., Kapteyn, H. C., Padmore, H. A., Lee, R. W., Wark, J. S., & Falcone, R. W. (2000). Time-Resolved X-Ray Diffraction from Coherent Phonons during a Laser-Induced Phase Transition. Physical Review Letters. https://doi.org/10.1103/physrevlett.84.111
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