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Mesoscopic Correlation of Supramolecular Chirality in One-Dimensional Hydrogen-Bonded Assemblies
Abstract
The ordering of 4-[trans-2-(pyrid-4-yl-vinyl)] benzoic acid, a two-dimensional chiral species, was studied by scanning tunneling microscopy at noble metal surfaces. Homochiral molecules self-assemble in supramolecular chiral hydrogen-bonded twin chains, which order in nanogratings where the supramolecular chirality is strictly correlated over the entire microm domains without intimate molecular contact. Model simulations indicate that the underlying mesoscopic chiral resolution is associated with twin chains acting as chiroselective templates for transient molecular attachment, which process mediates the gratings' evolution.
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Citations
Cites
Asymmetric Scattering of Polarized Electrons by Organized Organic Films of Chiral Molecules
Ray, K., Ananthavel, S. P., Waldeck, D. H., & Naaman, R. (1999) · Science · doi:10.1126/science.283.5403.814 · Cited by 613
Cited by
Supramolecular Chirality in Self-Assembled Systems
Liu, M., Zhang, L., & Wang, T. (2015) · Chemical Reviews · doi:10.1021/cr500671p · Cited by 2,250
Molecular Architectonic on Metal Surfaces
Barth, J. V. (2007) · Annual Review of Physical Chemistry · doi:10.1146/annurev.physchem.56.092503.141259 · Cited by 1,049
Self-citationSelf-Assembly at the Liquid/Solid Interface: STM Reveals
De Feyter, S., & De Schryver, F. C. (2005) · The Journal of Physical Chemistry B · doi:10.1021/jp045298k · Cited by 485
Tailoring molecular layers at metal surfaces
Bartels, L. (2010) · Nature Chemistry · doi:10.1038/nchem.517 · Cited by 451
Molecular chirality at surfaces
Ernst, K. (2012) · physica status solidi (b) · doi:10.1002/pssb.201248188 · Cited by 260
Metadata
- Authors
- Weckesser, J., De Vita, A., Barth, J. V., Cai, C., & Kern, K.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2001-08-09
- Volume
- 87
- Issue
- 9
- Pages
- 096101-096101
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2103308843
- Cited by
- 198
- References
- 1
- FWCI
- 10.48
- Type
- journal article
- Language
- en
- Open access
- closed
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- Weckesser, J., De Vita, A., Barth, J. V., Cai, C., & Kern, K. (2001). Mesoscopic Correlation of Supramolecular Chirality in One-Dimensional Hydrogen-Bonded Assemblies. Physical Review Letters. https://doi.org/10.1103/physrevlett.87.096101
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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