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Imaging Water Dissociation onTiO2(110)
Open accessAbstract
Scanning tunneling microscopy has been used to identify the adsorption site of ${\mathrm{H}}_{2}\mathrm{O}$ on ${\mathrm{TiO}}_{2}(110)\ensuremath{-}(1\ifmmode\times\else\texttimes\fi{}1)$ at 150 K, and to monitor the site of the dissociation products at 290 K. Water adsorbs onto the rows of fivefold coordinated Ti atoms at 150 K, dissociating by 290 K to form bridging but not terminal hydroxyls. This points to the involvement of bridging O vacancies in the dissociation pathway.
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Cited by
Titanium Dioxide Crystals with Tailored Facets
Liu, G., Yang, H. G., Pan, J., Yang, Y. Q., Lu, G. Q. (., & Cheng, H.-M. (2014) · Chemical Reviews · doi:10.1021/cr400621z · Cited by 1,084
Molecular Structure of Water at Interfaces: Wetting at the Nanometer Scale
Verdaguer, A., Sacha, G. M., Bluhm, H., & Salmeron, M. (2006) · Chemical Reviews · doi:10.1021/cr040376l · Cited by 627
Mechanism of H2O2 Decomposition on Transition Metal Oxide Surfaces
Lousada, C. M., Johansson, A. J., Brinck, T., & Jonsson, M. (2012) · The Journal of Physical Chemistry C · doi:10.1021/jp300255h · Cited by 286
Imanishi, A., Okamura, T., Ohashi, N., Nakamura, R., & Nakato, Y. (2007) · Journal of the American Chemical Society · doi:10.1021/ja073206+ · Cited by 254
Metadata
- Authors
- Brookes, I. M., Muryn, C. A., & Thornton, G.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2001-12-06
- Volume
- 87
- Issue
- 26
- Pages
- 266103-266103
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2075314982
- Cited by
- 338
- References
- 0
- FWCI
- 9.56
- Type
- journal article
- Language
- en
- Open access
- green
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