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Oxygen Vacancies as Active Sites for Water Dissociation on RutileTiO2(110)
Open accessAbstract
Through an interplay between scanning tunneling microscopy experiments and density functional theory calculations, we determine unambiguously the active surface site responsible for the dissociation of water molecules adsorbed on rutile TiO(2)(110). Oxygen vacancies in the surface layer are shown to dissociate H(2)O through the transfer of one proton to a nearby oxygen atom, forming two hydroxyl groups for every vacancy. The amount of water dissociation is limited by the density of oxygen vacancies present on the clean surface exclusively. The dissociation process sets in as soon as molecular water is able to diffuse to the active site.
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Citations
Cites
Photocatalysis on TiO2 Surfaces: Principles, Mechanisms, and Selected Results
Linsebigler, A. L., Lu, G., & Yates, J. T. (1995) · Chemical Reviews · doi:10.1021/cr00035a013 · Cited by 11,575
Cited by
The surface science of titanium dioxide
Diebold, U. (2003) · Surface Science Reports · doi:10.1016/s0167-5729(02)00100-0 · Cited by 7,944
TiO2 photocatalysis and related surface phenomena
FUJISHIMA, A., ZHANG, X., & TRYK, D. (2008) · Surface Science Reports · doi:10.1016/j.surfrep.2008.10.001 · Cited by 6,737
Surface Science Studies of the Photoactivation of TiO 2 New Photochemical Processes
Thompson, T. L., & Yates, J. T. (2006) · Chemical Reviews · doi:10.1021/cr050172k · Cited by 2,064
Oxygen Vacancy‐Mediated Photocatalysis of BiOCl: Reactivity, Selectivity, and Perspectives
Li, H., Li, J., Ai, Z., Jia, F., & Zhang, L. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201705628 · Cited by 1,207
Titanium Dioxide Crystals with Tailored Facets
Liu, G., Yang, H. G., Pan, J., Yang, Y. Q., Lu, G. Q. (., & Cheng, H.-M. (2014) · Chemical Reviews · doi:10.1021/cr400621z · Cited by 1,084
Metadata
- Authors
- Schaub, R., Thostrup, P., Lopez, N., Lægsgaard, E., Stensgaard, I., Nørskov, J. K., & Besenbacher, F.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2001-12-06
- Volume
- 87
- Issue
- 26
- Pages
- 266104-266104
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2139491573
- Cited by
- 997
- References
- 1
- FWCI
- 24.28
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Schaub, R., Thostrup, P., Lopez, N., Lægsgaard, E., Stensgaard, I., Nørskov, J. K., & Besenbacher, F. (2001). Oxygen Vacancies as Active Sites for Water Dissociation on RutileTiO2(110). Physical Review Letters. https://doi.org/10.1103/physrevlett.87.266104
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