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Phase Behavior in Thin Films of Cylinder-Forming Block Copolymers
Abstract
We have experimentally determined a phase diagram for cylinder-forming polystyrene-block-polybutadien-block-polystyrene triblock copolymer in thin films. The phase behavior can be modeled in great detail by dynamic density functional theory. Deviations from the bulk structure, such as wetting layer, perforated lamella, and lamella, are identified as surface reconstructions. Their stability regions are determined by an interplay between surface fields and confinement effects.
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Citations
Cites
The Physics of Block Copolymers
Hamley, I. W. (1998) · doi:10.1093/oso/9780198502180.001.0001 · Cited by 1,913
Cited by
Directing the self-assembly of block copolymers
Darling, S. B. (2007) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2007.05.004 · Cited by 1,019
Nanostructure fabrication using block copolymers
Hamley, I. W. (2003) · Nanotechnology · doi:10.1088/0957-4484/14/10/201 · Cited by 773
Solvent Vapor Annealing of Block Polymer Thin Films
Sinturel, C., Vayer, M., Morris, M., & Hillmyer, M. A. (2013) · Macromolecules · doi:10.1021/ma400735a · Cited by 543
Ma, M., Hill, R. M., Lowery, J. L., Fridrikh, S. V., & Rutledge, G. C. (2005) · Langmuir · doi:10.1021/la047064y · Cited by 494
(2007) · doi:10.1002/9783527610570.ch9 · Cited by 20
Metadata
- Authors
- Knoll, A., Horvat, A., Lyakhova, K. S., Krausch, G., Sevink, G. J. A., Zvelindovsky, A. V., & Magerle, R.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2002-06-27
- Volume
- 89
- Issue
- 3
- Pages
- 035501-035501
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2040997259
- Cited by
- 521
- References
- 1
- FWCI
- 13.80
- Type
- journal article
- Language
- en
- Open access
- closed
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- Knoll, A., Horvat, A., Lyakhova, K. S., Krausch, G., Sevink, G. J. A., Zvelindovsky, A. V., & Magerle, R. (2002). Phase Behavior in Thin Films of Cylinder-Forming Block Copolymers. Physical Review Letters. https://doi.org/10.1103/physrevlett.89.035501
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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