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Ultrafast Dephasing of Surface Plasmon Excitation in Silver Nanoparticles: Influence of Particle Size, Shape, and Chemical Surrounding
Abstract
By combination of two special methods, i.e., persistent spectral hole burning and laser assisted nanoparticle preparation, the dephasing time T2 of surface plasmon excitation in silver nanoparticles was systematically investigated. A strong dependence of T2 on the plasmon energy is found which reflects the relevance of interband damping and makes necessary a precise control of the particle shape when measuring T2. The influence of the reduced dimension on the dephasing dynamics was observed as a decrease of T2 with shrinking particle size. In addition, for silver nanoparticles on quartz substrates, a considerable amount of chemical interface damping was observed.
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Citations
Cited by
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Aslam, U., Rao, V. G., Chavez, S., & Linic, S. (2018) · Nature Catalysis · doi:10.1038/s41929-018-0138-x · Cited by 868
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Amendola, V., & Meneghetti, M. (2009) · The Journal of Physical Chemistry C · doi:10.1021/jp8082425 · Cited by 708
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Ma, X.-C., Dai, Y., Yu, L., & Huang, B.-B. (2016) · Light: Science & Applications · doi:10.1038/lsa.2016.17 · Cited by 553
Photochemistry on Metal Nanoparticles
Watanabe, K., Menzel, D., Nilius, N., & Freund, H.-J. (2006) · Chemical Reviews · doi:10.1021/cr050167g · Cited by 486
Metadata
- Authors
- Bosbach, J., Hendrich, C., Stietz, F., Vartanyan, T., & Träger, F.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2002-12-03
- Volume
- 89
- Issue
- 25
- Pages
- 257404-257404
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2054197087
- Cited by
- 174
- References
- 0
- FWCI
- 3.74
- Type
- journal article
- Language
- en
- Open access
- closed
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- Bosbach, J., Hendrich, C., Stietz, F., Vartanyan, T., & Träger, F. (2002). Ultrafast Dephasing of Surface Plasmon Excitation in Silver Nanoparticles: Influence of Particle Size, Shape, and Chemical Surrounding. Physical Review Letters. https://doi.org/10.1103/physrevlett.89.257404
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