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Structure and Bonding of Water on Pt(111)
Abstract
We address the adsorption of water on Pt(111) using x-ray absorption, x-ray emission, and x-ray photoelectron spectroscopy along with calculations in the framework of density functional theory. Using the direct relationship between the electronic structure and adsorbate geometry, we show that in the first layer all the molecules bind directly to the surface and to each other through the in-layer H bonds without dissociation, creating a nearly flat overlayer. The water molecules are adsorbed through alternating metal-oxygen (M-O) and metal-hydrogen (M-HO) bonds.
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Cited by
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Combining theory and experiment in electrocatalysis: Insights into materials design
Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F. (2017) · Science · doi:10.1126/science.aad4998 · Cited by 12,114
The Mechanism of Water Oxidation: From Electrolysis via Homogeneous to Biological Catalysis
Dau, H., Limberg, C., Reier, T., Risch, M., Roggan, S., & Strasser, P. (2010) · ChemCatChem · doi:10.1002/cctc.201000126 · Cited by 1,783
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Verdaguer, A., Sacha, G. M., Bluhm, H., & Salmeron, M. (2006) · Chemical Reviews · doi:10.1021/cr040376l · Cited by 627
Zhu, S., Qin, X., Xiao, F., Yang, S., Xu, Y., Tan, Z., Li, J., Yan, J., Chen, Q., Chen, M., et al. (2021) · Nature Catalysis · doi:10.1038/s41929-021-00663-5 · Cited by 436
Metadata
- Authors
- Ogasawara, H., Brena, B., Nordlund, D., Nyberg, M., Pelmenschikov, A., Pettersson, L. G. M., & Nilsson, A.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2002-12-18
- Volume
- 89
- Issue
- 27
- Pages
- 276102-276102
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2004731257
- Cited by
- 581
- References
- 0
- FWCI
- 18.97
- Type
- journal article
- Language
- en
- Open access
- closed
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- Ogasawara, H., Brena, B., Nordlund, D., Nyberg, M., Pelmenschikov, A., Pettersson, L. G. M., & Nilsson, A. (2002). Structure and Bonding of Water on Pt(111). Physical Review Letters. https://doi.org/10.1103/physrevlett.89.276102
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