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Multichromophoric Förster Resonance Energy Transfer
Abstract
The theory of Förster resonance energy transfer is generalized for multichromophoric (MC) and nonequilibrium situations. For the first time, it is clarified that the far-field linear spectroscopic information is insufficient for the determination of the reaction rate and that distance dependence of the rate can vary with the disorder and temperature. Application to a light harvesting complex LH2 reveals the important consequences of a MC structure.
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Cited by
Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems
Engel, G. S., Calhoun, T. R., Read, E. L., Ahn, T.-K., Mančal, T., Cheng, Y.-C., Blankenship, R. E., & Fleming, G. R. (2007) · Nature · doi:10.1038/nature05678 · Cited by 3,315
Environment-assisted quantum walks in photosynthetic energy transfer
Mohseni, M., Rebentrost, P., Lloyd, S., & Aspuru-Guzik, A. (2008) · The Journal of Chemical Physics · doi:10.1063/1.3002335 · Cited by 1,189
Coherent Two-Dimensional Optical Spectroscopy
Cho, M. (2008) · Chemical Reviews · doi:10.1021/cr078377b · Cited by 835
Ishizaki, A., & Fleming, G. R. (2009) · The Journal of Chemical Physics · doi:10.1063/1.3155372 · Cited by 734
Quantum entanglement in photosynthetic light-harvesting complexes
Sarovar, M., Ishizaki, A., Fleming, G. R., & Whaley, K. B. (2010) · Nature Physics · doi:10.1038/nphys1652 · Cited by 644
Metadata
- Authors
- Jang, S., Newton, M. D., & Silbey, R. J.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2004-05-25
- Volume
- 92
- Issue
- 21
- Pages
- 218301-218301
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2090061616
- Cited by
- 393
- References
- 0
- FWCI
- 6.76
- Type
- journal article
- Language
- en
- Open access
- closed
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