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Dynamical Singlets and Correlation-Assisted Peierls Transition inVO2
Open accessAbstract
A theory of the metal-insulator transition in vanadium dioxide from the high- temperature rutile to the low- temperature monoclinic phase is proposed on the basis of cluster dynamical mean-field theory, in conjunction with the density functional scheme. The interplay of strong electronic Coulomb interactions and structural distortions, in particular, the dimerization of vanadium atoms in the low-temperature phase, plays a crucial role. We find that VO2 is not a conventional Mott insulator, but that the formation of dynamical V-V singlet pairs due to strong Coulomb correlations is necessary to trigger the opening of a Peierls gap.
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Cited by
Mott Transition in VO 2 Revealed by Infrared Spectroscopy and Nano-Imaging
Qazilbash, M. M., Brehm, M., Chae, B.-G., Ho, P.-C., Andreev, G. O., Kim, B.-J., Yun, S. J., Balatsky, A. V., Maple, M. B., Keilmann, F., et al. (2007) · Science · doi:10.1126/science.1150124 · Cited by 1,539
Orbital-Assisted Metal-Insulator Transition inVO2
Haverkort, M. W., Hu, Z., Tanaka, A., Reichelt, W., Streltsov, S. V., Korotin, M. A., Anisimov, V. I., Hsieh, H. H., Lin, H.-J., Chen, C. T., et al. (2005) · Physical Review Letters · doi:10.1103/physrevlett.95.196404 · Cited by 409
Jager, M. F., Ott, C., Kraus, P. M., Kaplan, C. J., Pouse, W., Marvel, R. E., Haglund, R. F., Neumark, D. M., & Leone, S. R. (2017) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.1707602114 · Cited by 164
Metadata
- Authors
- Biermann, S., Poteryaev, A., Lichtenstein, A. I., & Georges, A.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2005-01-18
- Volume
- 94
- Issue
- 2
- Pages
- 026404-026404
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2064622618
- Cited by
- 715
- References
- 0
- FWCI
- 22.92
- Type
- journal article
- Language
- en
- Open access
- green
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- Biermann, S., Poteryaev, A., Lichtenstein, A. I., & Georges, A. (2005). Dynamical Singlets and Correlation-Assisted Peierls Transition inVO2. Physical Review Letters. https://doi.org/10.1103/physrevlett.94.026404
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