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New Information on Water Interfacial Structure Revealed by Phase-Sensitive Surface Spectroscopy
Abstract
A phase-sensitive sum-frequency vibrational spectroscopic technique is developed to study interfacial water structure of water/quartz interfaces. Measurements allow deduction of both real and imaginary parts of the surface nonlinear spectral response, revealing an unprecedentedly detailed picture of the net polar orientations of the water species at the interface. The orientations of the icelike and liquidlike species appear to respond very differently to the bulk pH change indicating the existence of different surface sites on quartz with different deprotonation pK values.
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Cited by
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Verdaguer, A., Sacha, G. M., Bluhm, H., & Salmeron, M. (2006) · Chemical Reviews · doi:10.1021/cr040376l · Cited by 627
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Wu, H., Li, X., Tung, C., & Wu, L. (2019) · Advanced Materials · doi:10.1002/adma.201900709 · Cited by 486
Hydrogen bonding at the water surface revealed by isotopic dilution spectroscopy
Stiopkin, I. V., Weeraman, C., Pieniazek, P. A., Shalhout, F. Y., Skinner, J. L., & Benderskii, A. V. (2011) · Nature · doi:10.1038/nature10173 · Cited by 462
Metadata
- Authors
- Ostroverkhov, V., Waychunas, G. A., & Shen, Y. R.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2005-02-02
- Volume
- 94
- Issue
- 4
- Pages
- 046102-046102
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2001443424
- Cited by
- 432
- References
- 0
- FWCI
- 13.73
- Type
- journal article
- Language
- en
- Open access
- closed
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- Ostroverkhov, V., Waychunas, G. A., & Shen, Y. R. (2005). New Information on Water Interfacial Structure Revealed by Phase-Sensitive Surface Spectroscopy. Physical Review Letters. https://doi.org/10.1103/physrevlett.94.046102
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