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Dynamics of Water Confined on a Nanometer Length Scale in Reverse Micelles: Ultrafast Infrared Vibrational Echo Spectroscopy
Abstract
The dynamics of water, confined on a nanometer length scale (1.7 to 4.0 nm) in sodium bis-(2-ethylhexyl) sulfosuccinate reverse micelles, is directly investigated using frequency resolved infrared vibrational echo experiments. The data are compared to bulk water and salt solution data. The experimentally determined frequency-frequency correlation functions show that the confined water dynamics is substantially slower than bulk water dynamics and is size dependent. The fastest dynamics (approximately 50 fs) is more similar to bulk water, while the slowest time scale dynamics is much slower than water, and, in analogy to bulk water, reflects the making and breaking of hydrogen bonds.
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Citations
Cited by
Hydrogen bond dynamics in aqueous NaBr solutions
Park, S., & Fayer, M. D. (2007) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.0707824104 · Cited by 313
Self-citationAnalysis of Water in Confined Geometries and at Interfaces
Fayer, M. D., & Levinger, N. E. (2010) · Annual Review of Analytical Chemistry · doi:10.1146/annurev-anchem-070109-103410 · Cited by 284
Self-citationConfinement or the Nature of the Interface? Dynamics of Nanoscopic Water
Moilanen, D. E., Levinger, N. E., Spry, D. B., & Fayer, M. D. (2007) · Journal of the American Chemical Society · doi:10.1021/ja073977d · Cited by 259
Self-citationFinite Size Effects on Hydrogen Bonds in Confined Water
Musat, R., Renault, J. P., Candelaresi, M., Palmer, D. J., Le Caër, S., Righini, R., & Pommeret, S. (2008) · Angewandte Chemie International Edition · doi:10.1002/anie.200802630 · Cited by 54
Qi, W., Chen, J., Yang, J., Lei, X., Song, B., & Fang, H. (2013) · The Journal of Physical Chemistry B · doi:10.1021/jp3120435 · Cited by 28
Metadata
- Authors
- Tan, H.-S., Piletic, I. R., Riter, R. E., Levinger, N. E., & Fayer, M. D.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2005-02-09
- Volume
- 94
- Issue
- 5
- Pages
- 057405-057405
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2169061898
- Cited by
- 164
- References
- 0
- FWCI
- 11.27
- Type
- journal article
- Language
- en
- Open access
- closed
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- Tan, H.-S., Piletic, I. R., Riter, R. E., Levinger, N. E., & Fayer, M. D. (2005). Dynamics of Water Confined on a Nanometer Length Scale in Reverse Micelles: Ultrafast Infrared Vibrational Echo Spectroscopy. Physical Review Letters. https://doi.org/10.1103/physrevlett.94.057405
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