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Reversible Thermoelectric Nanomaterials
Open accessAbstract
Irreversible effects in thermoelectric materials limit their efficiency and economy for applications in power generation and refrigeration. While electron transport is unavoidably irreversible in bulk materials, here we derive conditions under which reversible diffusive electron transport can be achieved in nanostructured thermoelectric materials. We provide a fundamental thermodynamic explanation for why the optimum density of states in a thermoelectric material is a delta function and for why inhomogeneous doping and segmentation improve the thermoelectric figure of merit.
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Citations
Cited by
Stochastic thermodynamics, fluctuation theorems and molecular machines
Seifert, U. (2012) · Reports on Progress in Physics · doi:10.1088/0034-4885/75/12/126001 · Cited by 3,300
Advances in thermoelectric materials research: Looking back and moving forward
He, J., & Tritt, T. M. (2017) · Science · doi:10.1126/science.aak9997 · Cited by 2,767
Silicon nanowires as efficient thermoelectric materials
Boukai, A. I., Bunimovich, Y., Tahir-Kheli, J., Yu, J.-K., Goddard III, W. A., & Heath, J. R. (2008) · Nature · doi:10.1038/nature06458 · Cited by 2,729
Nanostructured Thermoelectrics: Big Efficiency Gains from Small Features
Vineis, C. J., Shakouri, A., Majumdar, A., & Kanatzidis, M. G. (2010) · Advanced Materials · doi:10.1002/adma.201000839 · Cited by 1,430
Thermoelectricity in Molecular Junctions
Reddy, P., Jang, S.-Y., Segalman, R. A., & Majumdar, A. (2007) · Science · doi:10.1126/science.1137149 · Cited by 955
Metadata
- Authors
- Humphrey, T. E., & Linke, H.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2005-03-09
- Volume
- 94
- Issue
- 9
- Pages
- 096601-096601
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W4233235406
- Cited by
- 343
- References
- 0
- FWCI
- 9.27
- Type
- journal article
- Language
- en
- Open access
- green
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