The DOI matches its Crossref record; 25 of the 25 references it cites were found in a registry or an index.
Breaking the Phonon Bottleneck in Semiconductor Nanocrystals via Multiphonon Emission Induced by Intrinsic Nonadiabatic Interactions
Abstract
We observe ultrafast 1P-to-1S intraband relaxation in PbSe and CdSe nanocrystals (NCs) that have distinct energy spectra. While ultrafast dynamics in CdSe NCs has typically been interpreted in terms of electron-hole energy transfer, this mechanism is not active in PbSe NCs because of sparse densities of states in the conduction and valence bands. Our observations of temperature activation and confinement-enhanced relaxation in PbSe NCs can be explained by efficient multiphonon emission triggered by nonadiabatic electron-phonon interactions and are indicative of large, size-dependent, intraband Huang-Rhys parameters.
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Cites
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Cited by
Spectroscopic and Device Aspects of Nanocrystal Quantum Dots
Pietryga, J. M., Park, Y.-S., Lim, J., Fidler, A. F., Bae, W. K., Brovelli, S., & Klimov, V. I. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00169 · Cited by 1,040
Self-citationHot-Electron Transfer from Semiconductor Nanocrystals
Tisdale, W. A., Williams, K. J., Timp, B. A., Norris, D. J., Aydil, E. S., & Zhu, X.-Y. (2010) · Science · doi:10.1126/science.1185509 · Cited by 871
Makarov, N. S., Guo, S., Isaienko, O., Liu, W., Robel, I., & Klimov, V. I. (2016) · Nano Letters · doi:10.1021/acs.nanolett.5b05077 · Cited by 685
Self-citationColloidal quantum dot electronics
Liu, M., Yazdani, N., Yarema, M., Jansen, M., Wood, V., & Sargent, E. H. (2021) · Nature Electronics · doi:10.1038/s41928-021-00632-7 · Cited by 448
Kershaw, S. V., Susha, A. S., & Rogach, A. L. (2013) · Chemical Society Reviews · doi:10.1039/c2cs35331h · Cited by 433
Metadata
- Authors
- Schaller, R. D., Pietryga, J. M., Goupalov, S. V., Petruska, M. A., Ivanov, S. A., & Klimov, V. I.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2005-10-31
- Volume
- 95
- Issue
- 19
- Pages
- 196401-196401
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2031808719
- Cited by
- 270
- References
- 25
- FWCI
- 10.08
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Schaller, R. D., Pietryga, J. M., Goupalov, S. V., Petruska, M. A., Ivanov, S. A., & Klimov, V. I. (2005). Breaking the Phonon Bottleneck in Semiconductor Nanocrystals via Multiphonon Emission Induced by Intrinsic Nonadiabatic Interactions. Physical Review Letters. https://doi.org/10.1103/physrevlett.95.196401
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