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Relation between Dielectric and Low-Frequency Raman Spectra of Hydrogen-Bond Liquids
Open accessAbstract
We analyzed the complex dielectric and Raman spectra of hydrogen-bond liquids in the microwave to terahertz frequency range. As for water and methanol, the high-frequency component of the dielectric spectrum, i.e., the small deviation from the principal Debye relaxation, clearly corresponds to the Raman spectrum. This indicates that the cooperative relaxation, accompanied by huge polarization fluctuation, is virtually not Raman active, whereas the faster processes reflect common microscopic dynamics. For ethylene glycol, the shape of the Raman spectrum also resembles that of the high-frequency deviation of the dielectric spectrum, but, additionally, a weak manifestation of the cooperative relaxation arising from quadrupolar conformers is detected.
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Cited by
Intrinsic polymer dielectrics for high energy density and low loss electric energy storage
Wei, J., & Zhu, L. (2020) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2020.101254 · Cited by 328
Interactions and dynamics in electrolyte solutions by dielectric spectroscopy
Buchner, R., & Hefter, G. (2009) · Physical Chemistry Chemical Physics · doi:10.1039/b906555p · Cited by 318
Self-citationSmolyanskaya, O. A., Chernomyrdin, N. V., Konovko, A. A., Zaytsev, K. I., Ozheredov, I. A., Cherkasova, O. P., Nazarov, M. M., Guillet, J.-P., Kozlov, S. A., Kistenev, Y. V., et al. (2018) · Progress in Quantum Electronics · doi:10.1016/j.pquantelec.2018.10.001 · Cited by 292
Böhmer, R., Gainaru, C., & Richert, R. (2014) · Physics Reports · doi:10.1016/j.physrep.2014.07.005 · Cited by 280
Turton, D. A., Hunger, J., Stoppa, A., Hefter, G., Thoman, A., Walther, M., Buchner, R., & Wynne, K. (2009) · Journal of the American Chemical Society · doi:10.1021/ja903315v · Cited by 261
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Metadata
- Authors
- Fukasawa, T., Sato, T., Watanabe, J., Hama, Y., Kunz, W., & Buchner, R.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2005-11-03
- Volume
- 95
- Issue
- 19
- Pages
- 197802-197802
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2034425157
- Cited by
- 352
- References
- 0
- FWCI
- 3.83
- Type
- journal article
- Language
- en
- Open access
- green
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- Fukasawa, T., Sato, T., Watanabe, J., Hama, Y., Kunz, W., & Buchner, R. (2005). Relation between Dielectric and Low-Frequency Raman Spectra of Hydrogen-Bond Liquids. Physical Review Letters. https://doi.org/10.1103/physrevlett.95.197802
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