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Frequency-Dependent Spontaneous Emission Rate from CdSe and CdTe Nanocrystals: Influence of Dark States
Open accessAbstract
We studied the rate of spontaneous emission from colloidal CdSe and CdTe nanocrystals at room temperature. The decay rate, obtained from luminescence decay curves, increases with the emission frequency in a supralinear way. This dependence is explained by the thermal occupation of dark exciton states at room temperature, giving rise to a strong attenuation of the rate of emission. The supralinear dependence is in agreement with the results of tight-binding calculations.
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Citations
Cites
Controlling the dynamics of spontaneous emission from quantum dots by photonic crystals
Lodahl, P., Floris van Driel, A., Nikolaev, I. S., Irman, A., Overgaag, K., Vanmaekelbergh, D., & Vos, W. L. (2004) · Nature · doi:10.1038/nature02772 · Cited by 1,286
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Cited by
Size-Dependent Optical Properties of Colloidal PbS Quantum Dots
Moreels, I., Lambert, K., Smeets, D., De Muynck, D., Nollet, T., Martins, J. C., Vanhaecke, F., Vantomme, A., Delerue, C., Allan, G., et al. (2009) · ACS Nano · doi:10.1021/nn900863a · Cited by 1,249
Self-citationLuminescence in Sulfides: A Rich History and a Bright Future
Smet, P. F., Moreels, I., Hens, Z., & Poelman, D. (2010) · Materials · doi:10.3390/ma3042834 · Cited by 300
Lin, Z., Kohn, A. W., & Van Voorhis, T. (2020) · The Journal of Physical Chemistry C · doi:10.1021/acs.jpcc.9b08292 · Cited by 78
Kohn, A. W., Lin, Z., & Van Voorhis, T. (2019) · The Journal of Physical Chemistry C · doi:10.1021/acs.jpcc.9b01243 · Cited by 58
Metadata
- Authors
- van Driel, A. F., Allan, G., Delerue, C., Lodahl, P., Vos, W. L., & Vanmaekelbergh, D.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2005-12-01
- Volume
- 95
- Issue
- 23
- Pages
- 236804-236804
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2138451896
- Cited by
- 204
- References
- 1
- FWCI
- 6.45
- Type
- journal article
- Language
- en
- Open access
- green
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- van Driel, A. F., Allan, G., Delerue, C., Lodahl, P., Vos, W. L., & Vanmaekelbergh, D. (2005). Frequency-Dependent Spontaneous Emission Rate from CdSe and CdTe Nanocrystals: Influence of Dark States. Physical Review Letters. https://doi.org/10.1103/physrevlett.95.236804
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