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Enhancement and Quenching of Single-Molecule Fluorescence
Abstract
We present an experimental and theoretical study of the fluorescence rate of a single molecule as a function of its distance to a laser-irradiated gold nanoparticle. The local field enhancement leads to an increased excitation rate whereas nonradiative energy transfer to the particle leads to a decrease of the quantum yield (quenching). Because of these competing effects, previous experiments showed either fluorescence enhancement or fluorescence quenching. By varying the distance between molecule and particle we show the first experimental measurement demonstrating the continuous transition from fluorescence enhancement to fluorescence quenching. This transition cannot be explained by treating the particle as a polarizable sphere in the dipole approximation.
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Cites
Controlling the dynamics of spontaneous emission from quantum dots by photonic crystals
Lodahl, P., Floris van Driel, A., Nikolaev, I. S., Irman, A., Overgaag, K., Vanmaekelbergh, D., & Vos, W. L. (2004) · Nature · doi:10.1038/nature02772 · Cited by 1,286
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Tame, M. S., McEnery, K. R., Özdemir, Ş. K., Lee, J., Maier, S. A., & Kim, M. S. (2013) · Nature Physics · doi:10.1038/nphys2615 · Cited by 1,573
Probing the mechanisms of large Purcell enhancement in plasmonic nanoantennas
Akselrod, G. M., Argyropoulos, C., Hoang, T. B., Ciracì, C., Fang, C., Huang, J., Smith, D. R., & Mikkelsen, M. H. (2014) · Nature Photonics · doi:10.1038/nphoton.2014.228 · Cited by 1,084
Raman Techniques: Fundamentals and Frontiers
Jones, R. R., Hooper, D. C., Zhang, L., Wolverson, D., & Valev, V. K. (2019) · Nanoscale Research Letters · doi:10.1186/s11671-019-3039-2 · Cited by 804
MNPBEM—A Matlab toolbox for the simulation of plasmonic nanoparticles
Hohenester, U., & Trügler, A. (2012) · Computer Physics Communications · doi:10.1016/j.cpc.2011.09.009 · Cited by 798
Metadata
- Authors
- Anger, P., Bharadwaj, P., & Novotny, L.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2006-03-21
- Volume
- 96
- Issue
- 11
- Pages
- 113002-113002
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2023147957
- Cited by
- 3,158
- References
- 1
- FWCI
- 66.79
- Type
- journal article
- Language
- en
- Open access
- closed
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- Anger, P., Bharadwaj, P., & Novotny, L. (2006). Enhancement and Quenching of Single-Molecule Fluorescence. Physical Review Letters. https://doi.org/10.1103/physrevlett.96.113002
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
