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Control of the Charge State of Metal Atoms on Thin MgO Films
Open accessAbstract
The arrangement of single gold and palladium atoms deposited on the surface of a 3 monolayer thin film of MgO was investigated using low-temperature scanning tunneling microscopy. While Pd atoms are arranged in a random fashion, Au forms an ordered array on the surface. The long-range ordering as well as the scanning tunneling microscopy appearance of single Au atoms on a 3 monolayer thin MgO film can be explained by partial charge transfer from the substrate to Au atoms as predicted recently by density functional theory calculations [Phys. Rev. Lett. 94, 226104 (2005)10.1103/PhysRevLett.94.226104]. In contrast with that, Au atoms on a thick film were found to be essentially neutral.
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Citations
Cites
Charging Effects on Bonding and Catalyzed Oxidation of CO on Au 8 Clusters on MgO
Yoon, B., Häkkinen, H., Landman, U., Wörz, A. S., Antonietti, J.-M., Abbet, S., Judai, K., & Heiz, U. (2005) · Science · doi:10.1126/science.1104168 · Cited by 1,430
Cited by
Progress, Challenges, and Opportunities in Two-Dimensional Materials Beyond Graphene
Butler, S. Z., Hollen, S. M., Cao, L., Cui, Y., Gupta, J. A., Gutiérrez, H. R., Heinz, T. F., Hong, S. S., Huang, J., Ismach, A. F., et al. (2013) · ACS Nano · doi:10.1021/nn400280c · Cited by 4,878
Density functional theory for transition metals and transition metal chemistry
Cramer, C. J., & Truhlar, D. G. (2009) · Physical Chemistry Chemical Physics · doi:10.1039/b907148b · Cited by 1,648
Electronic interactions and charge transfers of metal atoms and clusters on oxide surfaces
Pacchioni, G. (2013) · Physical Chemistry Chemical Physics · doi:10.1039/c2cp43731g · Cited by 272
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Metadata
- Authors
- Sterrer, M., Risse, T., Martinez Pozzoni, U., Giordano, L., Heyde, M., Rust, H.-P., Pacchioni, G., & Freund, H.-J.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2007-03-02
- Volume
- 98
- Issue
- 9
- Pages
- 096107-096107
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2129236905
- Cited by
- 332
- References
- 1
- FWCI
- 19.76
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Sterrer, M., Risse, T., Martinez Pozzoni, U., Giordano, L., Heyde, M., Rust, H.-P., Pacchioni, G., & Freund, H.-J. (2007). Control of the Charge State of Metal Atoms on Thin MgO Films. Physical Review Letters. https://doi.org/10.1103/physrevlett.98.096107
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