The DOI matches its Crossref record; 6 of the 6 references it cites were found in a registry or an index.
Multi-principal elemental intermetallic nanoparticles synthesized via a disorder-to-order transition
Open accessAbstract
Nanoscale multi-principal element intermetallics (MPEIs) may provide a broad and tunable compositional space of active, high–surface area materials with potential applications such as catalysis and magnetics. However, MPEI nanoparticles are challenging to fabricate because of the tendency of the particles to grow/agglomerate or phase-separated during annealing. Here, we demonstrate a disorder-to-order phase transition approach that enables the synthesis of ultrasmall (4 to 5 nm) and stable MPEI nanoparticles (up to eight elements). We apply just 5 min of Joule heating to promote the phase transition of the nanoparticles into L1 0 intermetallic structure, which is then preserved by rapidly cooling. This disorder-to-order transition results in phase-stable nanoscale MPEIs with compositions (e.g., PtPdAuFeCoNiCuSn), which have not been previously attained by traditional synthetic methods. This synthesis strategy offers a new paradigm for developing previously unexplored MPEI nanoparticles by accessing a nanoscale-size regime and novel compositions with potentially broad applications.
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Cites
Monte Carlo sampling methods using Markov chains and their applications.
Hastings, W. K. (1970) · Biometrika · doi:10.1093/biomet/57.1.97 · Cited by 15,195
Monodisperse FePt Nanoparticles and Ferromagnetic FePt Nanocrystal Superlattices
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Self-citationXiong, Y., Yang, Y., Joress, H., Padgett, E., Gupta, U., Yarlagadda, V., Agyeman-Budu, D. N., Huang, X., Moylan, T. E., Zeng, R., et al. (2019) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.1815643116 · Cited by 173
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Self-citationTensile Strain-Mediated Spinel Ferrites Enable Superior Oxygen Evolution Activity
Yan, Y., Lin, J., Huang, K., Zheng, X., Qiao, L., Liu, S., Cao, J., Jun, S. C., Yamauchi, Y., & Qi, J. (2023) · Journal of the American Chemical Society · doi:10.1021/jacs.3c08598 · Cited by 294
High-entropy alloy electrocatalysts go to (sub-)nanoscale
Li, M., Lin, F., Zhang, S., Zhao, R., Tao, L., Li, L., Li, J., Zeng, L., Luo, M., & Guo, S. (2024) · Science Advances · doi:10.1126/sciadv.adn2877 · Cited by 177
Metadata
- Authors
- Cui, M., Yang, C., Hwang, S., Yang, M., Overa, S., Dong, Q., Yao, Y., Brozena, A. H., Cullen, D. A., Chi, M., Blum, T. F., Morris, D., Finfrock, Z., Wang, X., Zhang, P., Goncharov, V. G., Guo, X., Luo, J., Mo, Y., Jiao, F., & Hu, L.
- Venue
- Science Advances
- Published
- 2022-01-28
- Volume
- 8
- Issue
- 4
- Pages
- eabm4322-eabm4322
- ISSN
- 2375-2548 (ISSN-L)
- OpenAlex
- W4225071722
- Cited by
- 176
- References
- 6
- FWCI
- 13.93
- Type
- journal article
- Language
- en
- Open access
- gold
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- Cui, M., Yang, C., Hwang, S., Yang, M., Overa, S., Dong, Q., Yao, Y., Brozena, A. H., Cullen, D. A., Chi, M., Blum, T. F., Morris, D., Finfrock, Z., Wang, X., Zhang, P., Goncharov, V. G., Guo, X., Luo, J., Mo, Y., . . . Hu, L. (2022). Multi-principal elemental intermetallic nanoparticles synthesized via a disorder-to-order transition. Science Advances. https://doi.org/10.1126/sciadv.abm4322
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
