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Interwoven Metal-Organic Framework on a Periodic Minimal Surface with Extra-Large Pores
Abstract
Interpenetration (catenation) has long been considered a major impediment in the achievement of stable and porous crystalline structures. A strategy for the design of highly porous and structurally stable networks makes use of metal-organic building blocks that can be assembled on a triply periodic P -minimal geometric surface to produce structures that are interpenetrating—more accurately considered as interwoven. We used 4,4′,4"-benzene-1,3,5-triyl-tribenzoic acid (H 3 BTB), copper(II) nitrate, and N , N ′-dimethylformamide (DMF) to prepare Cu 3 (BTB) 2 (H 2 O) 3 ·(DMF) 9 (H 2 O) 2 (MOF-14), whose structure reveals a pair of interwoven metal-organic frameworks that are mutually reinforced. The structure contains remarkably large pores, 16.4 angstroms in diameter, in which voluminous amounts of gases and organic solvents can be reversibly sorbed.
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Cited by
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Davis, M. E. (2002) · Nature · doi:10.1038/nature00785 · Cited by 5,308
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Janiak, C. (2003) · Dalton Transactions · doi:10.1039/b305705b · Cited by 3,374
Dybtsev, D. N., Chun, H., & Kim, K. (2004) · Angewandte Chemie International Edition · doi:10.1002/anie.200460712 · Cited by 1,208
Metal–organic frameworks as a platform for clean energy applications
Li, X., Yang, X., Xue, H., Pang, H., & Xu, Q. (2020) · EnergyChem · doi:10.1016/j.enchem.2020.100027 · Cited by 706
Carné-Sánchez, A., Imaz, I., Cano-Sarabia, M., & Maspoch, D. (2013) · Nature Chemistry · doi:10.1038/nchem.1569 · Cited by 678
Metadata
- Authors
- Chen, B., Eddaoudi, M., Hyde, S. T., O'Keeffe, M., & Yaghi, O. M.
- Venue
- Science
- Published
- 2001-02-09
- Volume
- 291
- Issue
- 5506
- Pages
- 1021-1023
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2007203236
- Cited by
- 1,265
- References
- 0
- FWCI
- 54.81
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chen, B., Eddaoudi, M., Hyde, S. T., O'Keeffe, M., & Yaghi, O. M. (2001). Interwoven Metal-Organic Framework on a Periodic Minimal Surface with Extra-Large Pores. Science. https://doi.org/10.1126/science.1056598
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