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Stable Low-Pressure Hydrogen Clusters Stored in a Binary Clathrate Hydrate
Abstract
Thermodynamic, x-ray diffraction, and Raman and nuclear magnetic resonance spectroscopy measurements show that clusters of H 2 can be stabilized and stored at low pressures in a sII binary clathrate hydrate. Clusters of H 2 molecules occupy small water cages, whereas large water cages are singly occupied by tetrahydrofuran. The presence of this second guest component stabilizes the clathrate at pressures of 5 megapascals at 279.6 kelvin, versus 300 megapascals at 280 kelvin for pure H 2 hydrate.
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Citations
Cited by
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Preuster, P., Alekseev, A., & Wasserscheid, P. (2017) · Annual Review of Chemical and Biomolecular Engineering · doi:10.1146/annurev-chembioeng-060816-101334 · Cited by 486
Osman, A. I., Nasr, M., Eltaweil, A. S., Hosny, M., Farghali, M., Al-Fatesh, A. S., Rooney, D. W., & Abd El-Monaem, E. M. (2024) · International Journal of Hydrogen Energy · doi:10.1016/j.ijhydene.2024.03.223 · Cited by 270
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Metadata
- Authors
- Florusse, L. J., Peters, C. J., Schoonman, J., Hester, K. C., Koh, C. A., Dec, S. F., Marsh, K. N., & Sloan, E. D.
- Venue
- Science
- Published
- 2004-10-15
- Volume
- 306
- Issue
- 5695
- Pages
- 469-471
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2033416159
- Cited by
- 811
- References
- 0
- FWCI
- 23.35
- Type
- journal article
- Language
- en
- Open access
- closed
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- Florusse, L. J., Peters, C. J., Schoonman, J., Hester, K. C., Koh, C. A., Dec, S. F., Marsh, K. N., & Sloan, E. D. (2004). Stable Low-Pressure Hydrogen Clusters Stored in a Binary Clathrate Hydrate. Science. https://doi.org/10.1126/science.1102076
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