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Cation Exchange Reactions in Ionic Nanocrystals
Abstract
Cation exchange has been investigated in a wide range of nanocrystals of varying composition, size, and shape. Complete and fully reversible exchange occurs, and the rates of the reactions are much faster than in bulk cation exchange processes. A critical size has been identified below which the shapes of complex nanocrystals evolve toward the equilibrium shape with lowest energy during the exchange reaction. Above the critical size, the anion sublattice remains intact and the basic shapes of the initial nanocrystals are retained throughout the cation exchange. The size-dependent shape change can also be used to infer features of the microscopic mechanism.
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Cites
Shape control of CdSe nanocrystals
Peng, X., Manna, L., Yang, W., Wickham, J., Scher, E., Kadavanich, A., & Alivisatos, A. P. (2000) · Nature · doi:10.1038/35003535 · Cited by 4,487
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Gao, M.-R., Xu, Y.-F., Jiang, J., & Yu, S.-H. (2013) · Chemical Society Reviews · doi:10.1039/c2cs35310e · Cited by 1,610
Quantum Dots and Their Multimodal Applications: A Review
Bera, D., Qian, L., Tseng, T.-K., & Holloway, P. H. (2010) · Materials · doi:10.3390/ma3042260 · Cited by 1,365
Colloidal heterostructured nanocrystals: Synthesis and growth mechanisms
Carbone, L., & Cozzoli, P. D. (2010) · Nano Today · doi:10.1016/j.nantod.2010.08.006 · Cited by 691
CdSe nanocrystal based chem-/bio- sensors
Somers, R. C., Bawendi, M. G., & Nocera, D. G. (2007) · Chemical Society Reviews · doi:10.1039/b517613c · Cited by 616
High-Efficiency “Green” Quantum Dot Solar Cells
Pan, Z., Mora-Seró, I., Shen, Q., Zhang, H., Li, Y., Zhao, K., Wang, J., Zhong, X., & Bisquert, J. (2014) · Journal of the American Chemical Society · doi:10.1021/ja504310w · Cited by 608
Metadata
- Authors
- Son, D. H., Hughes, S. M., Yin, Y., & Paul Alivisatos, A.
- Venue
- Science
- Published
- 2004-11-05
- Volume
- 306
- Issue
- 5698
- Pages
- 1009-1012
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2007941671
- Cited by
- 1,277
- References
- 1
- FWCI
- 10.00
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
