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A Chromium Terephthalate-Based Solid with Unusually Large Pore Volumes and Surface Area
Open accessAbstract
We combined targeted chemistry and computational design to create a crystal structure for porous chromium terephthalate, MIL-101, withverylargeporesizes and surface area. Its zeotype cubic structure has a giant cell volume (∼702,000 cubic angstroms), a hierarchy of extra-large pore sizes (∼30 to 34 angstroms), and a Langmuir surface area for N 2 of ∼5900 ± 300 square meters per gram. Beside the usual properties of porous compounds, this solid has potential as a nanomold for monodisperse nanomaterials, as illustrated here by the incorporation of Keggin polyanions within the cages.
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Cited by
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Lee, J., Farha, O. K., Roberts, J., Scheidt, K. A., Nguyen, S. T., & Hupp, J. T. (2009) · Chemical Society Reviews · doi:10.1039/b807080f · Cited by 7,969
Metal–Organic Frameworks for Separations
Li, J.-R., Sculley, J., & Zhou, H.-C. (2012) · Chemical Reviews · doi:10.1021/cr200190s · Cited by 6,323
Valenzano, L., Civalleri, B., Chavan, S., Bordiga, S., Nilsen, M. H., Jakobsen, S., Lillerud, K. P., & Lamberti, C. (2011) · Chemistry of Materials · doi:10.1021/cm1022882 · Cited by 1,919
Perry IV, J. J., Perman, J. A., & Zaworotko, M. J. (2009) · Chemical Society Reviews · doi:10.1039/b807086p · Cited by 1,768
Synthesis and catalytic properties of MIL-100(Fe), an iron(iii) carboxylate with large pores
Horcajada, P., Surblé, S., Serre, C., Hong, D.-Y., Seo, Y.-K., Chang, J.-S., Grenèche, J.-M., Margiolaki, I., & Férey, G. (2007) · Chem. Commun. · doi:10.1039/b704325b · Cited by 1,538
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Metadata
- Authors
- Férey, G., Mellot-Draznieks, C., Serre, C., Millange, F., Dutour, J., Surblé, S., & Margiolaki, I.
- Venue
- Science
- Published
- 2005-09-23
- Volume
- 309
- Issue
- 5743
- Pages
- 2040-2042
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2007661885
- Cited by
- 5,430
- References
- 0
- FWCI
- 82.25
- Type
- journal article
- Language
- en
- Open access
- green
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- Férey, G., Mellot-Draznieks, C., Serre, C., Millange, F., Dutour, J., Surblé, S., & Margiolaki, I. (2005). A Chromium Terephthalate-Based Solid with Unusually Large Pore Volumes and Surface Area. Science. https://doi.org/10.1126/science.1116275
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