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Electrostatic Self-Assembly of Binary Nanoparticle Crystals with a Diamond-Like Lattice
Abstract
Self-assembly of charged, equally sized metal nanoparticles of two types (gold and silver) leads to the formation of large, sphalerite (diamond-like) crystals, in which each nanoparticle has four oppositely charged neighbors. Formation of these non–close-packed structures is a consequence of electrostatic effects specific to the nanoscale, where the thickness of the screening layer is commensurate with the dimensions of the assembling objects. Because of electrostatic stabilization of larger crystallizing particles by smaller ones, better-quality crystals can be obtained from more polydisperse nanoparticle solutions.
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Cited by
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Ghosh, S. K., & Pal, T. (2007) · Chemical Reviews · doi:10.1021/cr0680282 · Cited by 2,782
Bio‐Inspired, Smart, Multiscale Interfacial Materials
Xia, F., & Jiang, L. (2008) · Advanced Materials · doi:10.1002/adma.200800836 · Cited by 963
Thermodynamics versus Kinetics in Nanosynthesis
Wang, Y., He, J., Liu, C., Chong, W. H., & Chen, H. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201402986 · Cited by 497
Theoretical Studies of Plasmonics using Electronic Structure Methods
Morton, S. M., Silverstein, D. W., & Jensen, L. (2011) · Chemical Reviews · doi:10.1021/cr100265f · Cited by 474
Metadata
- Authors
- Kalsin, A. M., Fialkowski, M., Paszewski, M., Smoukov, S. K., Bishop, K. J. M., & Grzybowski, B. A.
- Venue
- Science
- Published
- 2006-04-21
- Volume
- 312
- Issue
- 5772
- Pages
- 420-424
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W1982308511
- Cited by
- 921
- References
- 0
- FWCI
- 40.34
- Type
- journal article
- Language
- en
- Open access
- closed
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- Kalsin, A. M., Fialkowski, M., Paszewski, M., Smoukov, S. K., Bishop, K. J. M., & Grzybowski, B. A. (2006). Electrostatic Self-Assembly of Binary Nanoparticle Crystals with a Diamond-Like Lattice. Science. https://doi.org/10.1126/science.1125124
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