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Isolated Single-Cycle Attosecond Pulses
Abstract
We generated single-cycle isolated attosecond pulses around ∼36 electron volts using phase-stabilized 5-femtosecond driving pulses with a modulated polarization state. Using a complete temporal characterization technique, we demonstrated the compression of the generated pulses for as low as 130 attoseconds, corresponding to less than 1.2 optical cycles. Numerical simulations of the generation process show that the carrier-envelope phase of the attosecond pulses is stable. The availability of single-cycle isolated attosecond pulses opens the way to a new regime in ultrafast physics, in which the strong-field electron dynamics in atoms and molecules is driven by the electric field of the attosecond pulses rather than by their intensity profile.
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Cites
Attosecond control of electronic processes by intense light fields
Baltuška, A., Udem, T., Uiberacker, M., Hentschel, M., Goulielmakis, E., Gohle, C., Holzwarth, R., Yakovlev, V. S., Scrinzi, A., Hänsch, T. W., et al. (2003) · Nature · doi:10.1038/nature01414 · Cited by 1,653
Cited by
Krausz, F., & Ivanov, M. (2009) · Reviews of Modern Physics · doi:10.1103/revmodphys.81.163 · Cited by 5,468
Real-time observation of valence electron motion
Goulielmakis, E., Loh, Z.-H., Wirth, A., Santra, R., Rohringer, N., Yakovlev, V. S., Zherebtsov, S., Pfeifer, T., Azzeer, A. M., Kling, M. F., et al. (2010) · Nature · doi:10.1038/nature09212 · Cited by 1,312
Schultze, M., Fieß, M., Karpowicz, N., Gagnon, J., Korbman, M., Hofstetter, M., Neppl, S., Cavalieri, A. L., Komninos, Y., Mercouris, T., et al. (2010) · Science · doi:10.1126/science.1189401 · Cited by 1,121
Ultrafast electron dynamics in phenylalanine initiated by attosecond pulses
Calegari, F., Ayuso, D., Trabattoni, A., Belshaw, L., De Camillis, S., Anumula, S., Frassetto, F., Poletto, L., Palacios, A., Decleva, P., et al. (2014) · Science · doi:10.1126/science.1254061 · Cited by 849
Self-citationWirth, A., Hassan, M. T., Grguraš, I., Gagnon, J., Moulet, A., Luu, T. T., Pabst, S., Santra, R., Alahmed, Z. A., Azzeer, A. M., et al. (2011) · Science · doi:10.1126/science.1210268 · Cited by 664
Metadata
- Authors
- Sansone, G., Benedetti, E., Calegari, F., Vozzi, C., Avaldi, L., Flammini, R., Poletto, L., Villoresi, P., Altucci, C., Velotta, R., Stagira, S., De Silvestri, S., & Nisoli, M.
- Venue
- Science
- Published
- 2006-10-20
- Volume
- 314
- Issue
- 5798
- Pages
- 443-446
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W1991801420
- Cited by
- 1,719
- References
- 1
- FWCI
- 72.81
- Type
- journal article
- Language
- en
- Open access
- closed
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- Sansone, G., Benedetti, E., Calegari, F., Vozzi, C., Avaldi, L., Flammini, R., Poletto, L., Villoresi, P., Altucci, C., Velotta, R., Stagira, S., De Silvestri, S., & Nisoli, M. (2006). Isolated Single-Cycle Attosecond Pulses. Science. https://doi.org/10.1126/science.1132838
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