The DOI matches its Crossref record; 21 of the 21 references it cites were found in a registry or an index.
Time-Resolved Dynamics in N 2 O 4 Probed Using High Harmonic Generation
Abstract
The attosecond time-scale electron-recollision process that underlies high harmonic generation has uncovered extremely rapid electronic dynamics in atoms and diatomics. We showed that high harmonic generation can reveal coupled electronic and nuclear dynamics in polyatomic molecules. By exciting large amplitude vibrations in dinitrogen tetraoxide, we showed that tunnel ionization accesses the ground state of the ion at the outer turning point of the vibration but populates the first excited state at the inner turning point. This state-switching mechanism is manifested as bursts of high harmonic light that is emitted mostly at the outer turning point. Theoretical calculations attribute the large modulation to suppressed emission from the first excited state of the ion. More broadly, these results show that high harmonic generation and strong-field ionization in polyatomic molecules undergoing bonding or configurational changes involve the participation of multiple molecular orbitals.
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Cites
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Cited by
High harmonic interferometry of multi-electron dynamics in molecules
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Self-citationAttosecond imaging of molecular electronic wavepackets
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Spin angular momentum and tunable polarization in high-harmonic generation
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Imaging ultrafast molecular dynamics with laser-induced electron diffraction
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Generation of bright phase-matched circularly-polarized extreme ultraviolet high harmonics
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Metadata
- Authors
- Li, W., Zhou, X., Lock, R., Patchkovskii, S., Stolow, A., Kapteyn, H. C., & Murnane, M. M.
- Venue
- Science
- Published
- 2008-11-21
- Volume
- 322
- Issue
- 5905
- Pages
- 1207-1211
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2064917327
- Cited by
- 351
- References
- 21
- FWCI
- 15.28
- Type
- journal article
- Language
- en
- Open access
- closed
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