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A Fast Soluble Carbon-Free Molecular Water Oxidation Catalyst Based on Abundant Metals
Abstract
Bulking Up Water Oxidation: Storing solar energy by water oxidation, in a process akin to photosynthesis, is a promising approach for building a renewable energy infrastructure. Unfortunately, many of the most active synthetic catalysts for this process fall prey to degradation by the generated oxygen. Yin et al. (p. 342 , published online 11 March; see the Perspective by Hurst ) used bulky polyoxometalate ligands to protect a catalytic cobalt center from this fate. The full complex was easily prepared by mixing proper ratios of inexpensive tungsten, cobalt, and phosphate salts in boiling water. After isolating and redissolving the catalyst in slightly basic aqueous solution, rapid oxygen generation was observed with a ruthenium-based oxidant.
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Cited by
Homogeneously dispersed multimetal oxygen-evolving catalysts
Zhang, B., Zheng, X., Voznyy, O., Comin, R., Bajdich, M., García-Melchor, M., Han, L., Xu, J., Liu, M., Zheng, L., et al. (2016) · Science · doi:10.1126/science.aaf1525 · Cited by 2,447
Chatenet, M., Pollet, B. G., Dekel, D. R., Dionigi, F., Deseure, J., Millet, P., Braatz, R. D., Bazant, M. Z., Eikerling, M., Staffell, I., et al. (2022) · Chemical Society Reviews · doi:10.1039/d0cs01079k · Cited by 2,025
The Mechanism of Water Oxidation: From Electrolysis via Homogeneous to Biological Catalysis
Dau, H., Limberg, C., Reier, T., Risch, M., Roggan, S., & Strasser, P. (2010) · ChemCatChem · doi:10.1002/cctc.201000126 · Cited by 1,783
A molecular ruthenium catalyst with water-oxidation activity comparable to that of photosystem II
Duan, L., Bozoglian, F., Mandal, S., Stewart, B., Privalov, T., Llobet, A., & Sun, L. (2012) · Nature Chemistry · doi:10.1038/nchem.1301 · Cited by 1,257
Recent Progress on Multimetal Oxide Catalysts for the Oxygen Evolution Reaction
Kim, J. S., Kim, B., Kim, H., & Kang, K. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201702774 · Cited by 940
Metadata
- Authors
- Yin, Q., Tan, J. M., Besson, C., Geletii, Y. V., Musaev, D. G., Kuznetsov, A. E., Luo, Z., Hardcastle, K. I., & Hill, C. L.
- Venue
- Science
- Published
- 2010-04-16
- Volume
- 328
- Issue
- 5976
- Pages
- 342-345
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2011715705
- Cited by
- 1,438
- References
- 0
- FWCI
- 57.15
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yin, Q., Tan, J. M., Besson, C., Geletii, Y. V., Musaev, D. G., Kuznetsov, A. E., Luo, Z., Hardcastle, K. I., & Hill, C. L. (2010). A Fast Soluble Carbon-Free Molecular Water Oxidation Catalyst Based on Abundant Metals. Science. https://doi.org/10.1126/science.1185372
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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