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Large-Area Three-Dimensional Molecular Ordering of a Polymer Brush by One-Step Processing
Abstract
Bend It, Stretch It: Materials (such as those found in some artificial muscle systems) that are used for stimulus-controlled bending or stretching, require long-range ordering so that local chemical triggers will result in long-range bending or flexing motions. Hosono et al. (p. 808 ) observed that a sandwich of a polymethacrylate between uniaxially stretched Teflon sheets develops three-dimensional ordering. Upon hot pressing, the main chains of the polymer brushes aligned homeotropically to the film plane, whereas the side chains, containing azobenzene groups, oriented horizontally along the drawing direction of the Teflon sheets. With some azobenzene groups, alternate irradiation with ultraviolet and visible light made the composites bend and stretch reversibly.
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Cited by
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Arazoe, H., Miyajima, D., Akaike, K., Araoka, F., Sato, E., Hikima, T., Kawamoto, M., & Aida, T. (2016) · Nature Materials · doi:10.1038/nmat4693 · Cited by 435
Self-citationProbing ultrafast ππ*/nπ* internal conversion in organic chromophores via K-edge resonant absorption
Wolf, T. J. A., Myhre, R. H., Cryan, J. P., Coriani, S., Squibb, R. J., Battistoni, A., Berrah, N., Bostedt, C., Bucksbaum, P., Coslovich, G., et al. (2017) · Nature Communications · doi:10.1038/s41467-017-00069-7 · Cited by 197
Light-triggered topological programmability in a dynamic covalent polymer network
Zou, W., Jin, B., Wu, Y., Song, H., Luo, Y., Huang, F., Qian, J., Zhao, Q., & Xie, T. (2020) · Science Advances · doi:10.1126/sciadv.aaz2362 · Cited by 143
Metadata
- Authors
- Hosono, N., Kajitani, T., Fukushima, T., Ito, K., Sasaki, S., Takata, M., & Aida, T.
- Venue
- Science
- Published
- 2010-11-05
- Volume
- 330
- Issue
- 6005
- Pages
- 808-811
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W1998971107
- Cited by
- 178
- References
- 0
- FWCI
- 6.59
- Type
- journal article
- Language
- en
- Open access
- closed
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- Hosono, N., Kajitani, T., Fukushima, T., Ito, K., Sasaki, S., Takata, M., & Aida, T. (2010). Large-Area Three-Dimensional Molecular Ordering of a Polymer Brush by One-Step Processing. Science. https://doi.org/10.1126/science.1195302
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