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Large-Pore Apertures in a Series of Metal-Organic Frameworks
Abstract
Maximizing Molecular Pore Diameters: Amorphous materials, such as activated carbon, can have pore diameters of several nanometers, but the synthesis of ordered structures with very large pore diameters is often thwarted by the creation of interpenetrating networks or difficulties in removing guest molecules. Deng et al. (p. 1018 ) avoided these problems in the synthesis of metal-organic frameworks (MOFs) with very large diameters (some exceeding 3 nanometers) by using a combination of short and very long linking groups. The compounds formed channels almost 10 nanometers in diameter that could be visualized by electron microscopy and that were large enough to accommodate protein molecules.
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Cited by
Metal–Organic Frameworks for Drug Delivery: A Design Perspective
Lawson, H. D., Walton, S. P., & Chan, C. (2021) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.1c01089 · Cited by 916
Metal–organic frameworks based on flexible ligands (FL-MOFs): structures and applications
Lin, Z.-J., Lü, J., Hong, M., & Cao, R. (2014) · Chem. Soc. Rev. · doi:10.1039/c3cs60483g · Cited by 874
Nanoconfined phase change materials for thermal energy applications
Aftab, W., Huang, X., Wu, W., Liang, Z., Mahmood, A., & Zou, R. (2018) · Energy & Environmental Science · doi:10.1039/c7ee03587j · Cited by 647
Understanding the diversity of the metal-organic framework ecosystem
Moosavi, S. M., Nandy, A., Jablonka, K. M., Ongari, D., Janet, J. P., Boyd, P. G., Lee, Y., Smit, B., & Kulik, H. J. (2020) · Nature Communications · doi:10.1038/s41467-020-17755-8 · Cited by 622
Luo, F., Yan, C., Dang, L., Krishna, R., Zhou, W., Wu, H., Dong, X., Han, Y., Hu, T.-L., O’Keeffe, M., et al. (2016) · Journal of the American Chemical Society · doi:10.1021/jacs.6b02030 · Cited by 601
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Metadata
- Authors
- Deng, H., Grunder, S., Cordova, K. E., Valente, C., Furukawa, H., Hmadeh, M., Gándara, F., Whalley, A. C., Liu, Z., Asahina, S., Kazumori, H., O’Keeffe, M., Terasaki, O., Stoddart, J. F., & Yaghi, O. M.
- Venue
- Science
- Published
- 2012-05-25
- Volume
- 336
- Issue
- 6084
- Pages
- 1018-1023
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W1996369650
- Cited by
- 2,126
- References
- 0
- FWCI
- 76.74
- Type
- journal article
- Language
- en
- Open access
- closed
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- Deng, H., Grunder, S., Cordova, K. E., Valente, C., Furukawa, H., Hmadeh, M., Gándara, F., Whalley, A. C., Liu, Z., Asahina, S., Kazumori, H., O’Keeffe, M., Terasaki, O., Stoddart, J. F., & Yaghi, O. M. (2012). Large-Pore Apertures in a Series of Metal-Organic Frameworks. Science. https://doi.org/10.1126/science.1220131
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