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Titanium and Zinc Oxide Nanoparticles Are Proton-Coupled Electron Transfer Agents
Abstract
Pluses and Minuses: Because of their high surface area and tunable electronic structure, nanoparticles are of interest for next-generation photocatalysis and light-harvesting applications. Many of these applications involve electron transfer events at the particle surface after light absorption. Schrauben et al. (p. 1298 ) now show, through a series of radical trap kinetic studies, that proton transfer can concurrently accompany electron transfer at the solvent interfaces of two common nanoparticle formulations (oxides of titanium and of zinc). The results may help in the optimization of particle structure and energetics.
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Cited by
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Agrawal, A., Cho, S. H., Zandi, O., Ghosh, S., Johns, R. W., & Milliron, D. J. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.7b00613 · Cited by 1,014
He, W., Kim, H.-K., Wamer, W. G., Melka, D., Callahan, J. H., & Yin, J.-J. (2014) · Journal of the American Chemical Society · doi:10.1021/ja410800y · Cited by 850
Zhao, Y., Chen, G., Bian, T., Zhou, C., Waterhouse, G. I. N., Wu, L., Tung, C., Smith, L. J., O'Hare, D., & Zhang, T. (2015) · Advanced Materials · doi:10.1002/adma.201503730 · Cited by 766
Selective Aerobic Oxidation Mediated by TiO2 Photocatalysis
Lang, X., Ma, W., Chen, C., Ji, H., & Zhao, J. (2014) · Accounts of Chemical Research · doi:10.1021/ar4001108 · Cited by 288
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Kitcatt, D. M., Nicolle, S., & Lee, A.-L. (2022) · Chemical Society Reviews · doi:10.1039/d1cs01168e · Cited by 257
Metadata
- Authors
- Schrauben, J. N., Hayoun, R., Valdez, C. N., Braten, M., Fridley, L., & Mayer, J. M.
- Venue
- Science
- Published
- 2012-06-08
- Volume
- 336
- Issue
- 6086
- Pages
- 1298-1301
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W1980602646
- Cited by
- 402
- References
- 0
- FWCI
- 12.51
- Type
- journal article
- Language
- en
- Open access
- closed
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- Schrauben, J. N., Hayoun, R., Valdez, C. N., Braten, M., Fridley, L., & Mayer, J. M. (2012). Titanium and Zinc Oxide Nanoparticles Are Proton-Coupled Electron Transfer Agents. Science. https://doi.org/10.1126/science.1220234
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
