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Direct Measurements of Conformer-Dependent Reactivity of the Criegee Intermediate CH 3 CHOO
Open accessAbstract
More Criegee Sightings: The reaction of ozone with unsaturated hydrocarbons produces short-lived molecules termed Criegee intermediates. The simplest such molecule, H 2 CO 2 , was recently detected and monitored in the laboratory. Su et al. (p. 174 ; see the Perspective by Vereecken ) have obtained its vibrational spectrum, which could ultimately enable direct measurements of its reactivity in the atmosphere. Taatjes et al. (p. 177 ; see the Perspective by Vereecken ) report on the laboratory preparation and reactivity of the next heavier Criegee intermediate, which bears a methyl group in place of one of the hydrogen atoms.
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Cites
New perspectives in multireference perturbation theory: the n-electron valence state approach
Angeli, C., Pastore, M., & Cimiraglia, R. (2007) · Theoretical Chemistry Accounts · doi:10.1007/s00214-006-0207-0 · Cited by 281
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Pöschl, U., & Shiraiwa, M. (2015) · Chemical Reviews · doi:10.1021/cr500487s · Cited by 657
The Molecular Identification of Organic Compounds in the Atmosphere: State of the Art and Challenges
Nozière, B., Kalberer, M., Claeys, M., Allan, J., D’Anna, B., Decesari, S., Finessi, E., Glasius, M., Grgić, I., Hamilton, J. F., et al. (2015) · Chemical Reviews · doi:10.1021/cr5003485 · Cited by 656
Taatjes, C. A., Khan, M. A. H., Eskola, A. J., Percival, C. J., Osborn, D. L., Wallington, T. J., & Shallcross, D. E. (2019) · Environmental Science & Technology · doi:10.1021/acs.est.8b05073 · Cited by 38
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Metadata
- Authors
- Taatjes, C. A., Welz, O., Eskola, A. J., Savee, J. D., Scheer, A. M., Shallcross, D. E., Rotavera, B., Lee, E. P. F., Dyke, J. M., Mok, D. K. W., Osborn, D. L., & Percival, C. J.
- Venue
- Science
- Published
- 2013-04-12
- Volume
- 340
- Issue
- 6129
- Pages
- 177-180
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W1995673006
- Cited by
- 457
- References
- 1
- FWCI
- 26.61
- Type
- journal article
- Language
- en
- Open access
- green
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- Taatjes, C. A., Welz, O., Eskola, A. J., Savee, J. D., Scheer, A. M., Shallcross, D. E., Rotavera, B., Lee, E. P. F., Dyke, J. M., Mok, D. K. W., Osborn, D. L., & Percival, C. J. (2013). Direct Measurements of Conformer-Dependent Reactivity of the Criegee Intermediate CH 3 CHOO. Science. https://doi.org/10.1126/science.1234689
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