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Reaction of O 2 with Subsurface Oxygen Vacancies on TiO 2 Anatase (101)
Open accessAbstract
Oxide Chemistry Below the Surface: Although metal oxides, such as titanium dioxide (TiO 2 ), are used for catalytic oxidation reactions and photocatalysis, the O 2 does not react directly with substrates. Vacancies in the surface region of the TiO 2 rutile phase can transfer a negative charge to adsorbed O 2 to create more reactive species. By contrast, in anatase—the phase associated with nanoscale TiO 2 particles—subsurface vacancies form. Setvin et al. (p. 988 ) used a scanning tunneling microscopy tip to pull these vacancies to the surface in a niobiumdoped anatase crystal and followed the transformation of adsorbed O 2 − into a peroxo species and a bridging O 2 dimer.
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Citations
Cites
Photocatalysis on TiO2 Surfaces: Principles, Mechanisms, and Selected Results
Linsebigler, A. L., Lu, G., & Yates, J. T. (1995) · Chemical Reviews · doi:10.1021/cr00035a013 · Cited by 11,575
The surface science of titanium dioxide
Diebold, U. (2003) · Surface Science Reports · doi:10.1016/s0167-5729(02)00100-0 · Cited by 7,944
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Cited by
Why is anatase a better photocatalyst than rutile? - Model studies on epitaxial TiO2 films
Luttrell, T., Halpegamage, S., Tao, J., Kramer, A., Sutter, E., & Batzill, M. (2014) · Scientific Reports · doi:10.1038/srep04043 · Cited by 1,544
Titanium Dioxide Crystals with Tailored Facets
Liu, G., Yang, H. G., Pan, J., Yang, Y. Q., Lu, G. Q. (., & Cheng, H.-M. (2014) · Chemical Reviews · doi:10.1021/cr400621z · Cited by 1,084
The roles of oxygen vacancies in electrocatalytic oxygen evolution reaction
Zhu, K., Shi, F., Zhu, X., & Yang, W. (2020) · Nano Energy · doi:10.1016/j.nanoen.2020.104761 · Cited by 1,018
Oxygen vacancies in metal oxides: recent progress towards advanced catalyst design
Zhuang, G., Chen, Y., Zhuang, Z., Yu, Y., & Yu, J. (2020) · Science China Materials · doi:10.1007/s40843-020-1305-6 · Cited by 499
Surface point defects on bulk oxides: atomically-resolved scanning probe microscopy
Setvín, M., Wagner, M., Schmid, M., Parkinson, G. S., & Diebold, U. (2017) · Chemical Society Reviews · doi:10.1039/c7cs00076f · Cited by 134
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Metadata
- Authors
- Setvín, M., Aschauer, U., Scheiber, P., Li, Y.-F., Hou, W., Schmid, M., Selloni, A., & Diebold, U.
- Venue
- Science
- Published
- 2013-08-30
- Volume
- 341
- Issue
- 6149
- Pages
- 988-991
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2069099421
- Cited by
- 565
- References
- 2
- FWCI
- 15.03
- Type
- journal article
- Language
- en
- Open access
- green
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- Setvín, M., Aschauer, U., Scheiber, P., Li, Y.-F., Hou, W., Schmid, M., Selloni, A., & Diebold, U. (2013). Reaction of O 2 with Subsurface Oxygen Vacancies on TiO 2 Anatase (101). Science. https://doi.org/10.1126/science.1239879
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