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Recyclable, Strong Thermosets and Organogels via Paraformaldehyde Condensation with Diamines
Abstract
Recyclable Thermoset Polymers: The high mechanical strength and durability of thermoset polymers are exploited in applications such as composite materials, where they form the matrix surrounding carbon fibers. The thermally driven polymerization reaction is usually irreversible, so it is difficult to recycle the constituent monomers and to remove and repair portions of a composite part. García et al. (p. 732 ; see the Perspective by Long ) now describe a family of polymers formed by condensation of paraformaldehyde with bisanilines that could form hard thermoset polymers or, when more oxygenated, produce self-healing gels. Strong acid digestion allowed recovery of the bisaniline monomers.
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Cites
Density-functional thermochemistry. III. The role of exact exchange
Becke, A. D. (1993) · The Journal of Chemical Physics · doi:10.1063/1.464913 · Cited by 103,767
Lee, C., Yang, W., & Parr, R. G. (1988) · Physical Review B · doi:10.1103/physrevb.37.785 · Cited by 100,874
Cited by
Chemical recycling of waste plastics for new materials production
Rahimi, A., & García, J. M. (2017) · Nature Reviews Chemistry · doi:10.1038/s41570-017-0046 · Cited by 2,121
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Lopez, J., Mackanic, D. G., Cui, Y., & Bao, Z. (2019) · Nature Reviews Materials · doi:10.1038/s41578-019-0103-6 · Cited by 894
Chemically recyclable polymers: a circular economy approach to sustainability
Hong, M., & Chen, E. Y.-X. (2017) · Green Chemistry · doi:10.1039/c7gc01496a · Cited by 876
A synthetic polymer system with repeatable chemical recyclability
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Closed-loop recycling of plastics enabled by dynamic covalent diketoenamine bonds
Christensen, P. R., Scheuermann, A. M., Loeffler, K. E., & Helms, B. A. (2019) · Nature Chemistry · doi:10.1038/s41557-019-0249-2 · Cited by 676
Metadata
- Authors
- García, J. M., Jones, G. O., Virwani, K., McCloskey, B. D., Boday, D. J., ter Huurne, G. M., Horn, H. W., Coady, D. J., Bintaleb, A. M., Alabdulrahman, A. M. S., Alsewailem, F., Almegren, H. A. A., & Hedrick, J. L.
- Venue
- Science
- Published
- 2014-05-16
- Volume
- 344
- Issue
- 6185
- Pages
- 732-735
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2112047597
- Cited by
- 472
- References
- 2
- FWCI
- 17.26
- Type
- journal article
- Language
- en
- Open access
- closed
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- García, J. M., Jones, G. O., Virwani, K., McCloskey, B. D., Boday, D. J., ter Huurne, G. M., Horn, H. W., Coady, D. J., Bintaleb, A. M., Alabdulrahman, A. M. S., Alsewailem, F., Almegren, H. A. A., & Hedrick, J. L. (2014). Recyclable, Strong Thermosets and Organogels via Paraformaldehyde Condensation with Diamines. Science. https://doi.org/10.1126/science.1251484
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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