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Conducting Carbon Wires in Ordered, Nanometer-Sized Channels
Open accessAbstract
The encapsulation of graphite-type carbon wires in the regular, 3-nanometer-wide hexagonal channels of the mesoporous host MCM-41 is reported. Acrylonitrile monomers are introduced through vapor or solution transfer and polymerized in the channels with external radical initiators. Pyrolysis of the intrachannel polyacrylonitrile results in filaments whose microwave conductivity is about 10 times that of bulk carbonized polyacrylonitrile. The MCM host plays a key role in ordering the carbon structure, most likely through the parallel alignment of the precursor polymer chains in the channels. The fabrication of stable carbon filaments in ordered, nanometer-sized channels represents an important step toward the development of nanometer electronics.
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Citations
Cited by
Mesoporous carbon materials: Synthesis and modification
Liang, C., Li, Z., & Dai, S. (2008) · Angewandte Chemie International Edition · doi:10.1002/anie.200702046 · Cited by 1,935
Ciesla, U., & Schüth, F. (1999) · Microporous and Mesoporous Materials · doi:10.1016/s1387-1811(98)00249-2 · Cited by 1,084
Inclusion Chemistry in Periodic Mesoporous Hosts
Moller, K., & Bein, T. (1998) · Chemistry of Materials · doi:10.1021/cm980243e · Cited by 916
Self-citationSOMC@PMS. Surface Organometallic Chemistry at Periodic Mesoporous Silica
Anwander, R. (2001) · Chemistry of Materials · doi:10.1021/cm0111534 · Cited by 320
Satoh, K., & Kamigaito, M. (2009) · Chemical Reviews · doi:10.1021/cr900115u · Cited by 302
Metadata
- Authors
- Wu, C.-G., & Bein, T.
- Venue
- Science
- Published
- 1994-11-11
- Volume
- 266
- Issue
- 5187
- Pages
- 1013-1015
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2062719459
- Cited by
- 372
- References
- 0
- FWCI
- 11.08
- Type
- journal article
- Language
- en
- Open access
- green
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